Controlling Quantum Spin States and Dynamics with Light

Coupling many atoms to a single mode of light provides an efficient means of generating quantum correlations in an extended many-body system. I will report on experiments in which we harness photons in an optical cavity to mediate “flip-flop” interactions among distant spins in a millimeter-long cloud of atoms, as we directly observe by imaging quench dynamics. In our spin-1 system, these exchange interactions enable correlated pair creation in the m = ±1 Zeeman states, a process analogous to spontaneous parametric down-conversion or to collisional spin mixing in Bose-Einstein condensates. In contrast to direct collisional interactions, non-local light-mediated interactions offer unprecedented opportunities for engineering the spatial structure of spin-spin couplings and correlations. I will describe progress and prospects in tailoring atom-light interactions to enable new directions in quantum simulation and to generate new resources for quantum-enhanced sensing.