Determining lattice distortion of Ba2NaOsO6

ORAL

Abstract

Exotic quantum phases have been proposed in magnetic Mott insulators with strong spin-orbit coupling. Our recent nuclear magnetic resonance (NMR) studies of the Mott insulator Ba2NaOsO6 established that local lattice distortions precede the onset of canted ferromagnetic order1,2. It was suggested that lattice distortions are a manifestation of the orbital order that drives the magnetism in this class of materials3. To decipher the microscopic nature of the putative orbital order, we investigate different lattice distortion models and calculate their associated NMR observables. Results of various distortion models will be discussed in this talk.

[1] Lu, L., et al. "Magnetism and local symmetry breaking in a Mott insulator with strong spin orbit interactions." Nature communications 8 (2017): 14407.
[2] Liu, W., et al. "Nature of lattice distortions in the cubic double perovskite Ba 2 NaOsO 6." Physical Review B 97.22 (2018): 224103.
[3] Chen, Gang, Rodrigo Pereira, and Leon Balents. "Exotic phases induced by strong spin-orbit coupling in ordered double perovskites." Physical Review B 82.17 (2010): 174440.

Presenters

  • Rong Cong

    Brown University

Authors

  • Rong Cong

    Brown University

  • Ravindra Nanguneri

    Brown University

  • Vesna F Mitrovic

    Brown University

  • Brenda Rubenstein

    Department of Chemistry, Brown University, Brown University