Synthesis and stability of thin films of purported skyrmion lattice metal SrFeO<sub>3</sub>

ORAL

Abstract

Solid state systems possessing non-trivial topological properties are of interest in the context of spintronic applications as well as the fundamental study of quantum materials with a Berry phase. A particularly fascinating example of such a system is the correlated oxide strontium ferrite, SrFeO3, due to its persistent metallicity and plethora of magnetic phases that arise from the high symmetry of its crystal structure 1. One type of multi-q spin structure is suggested to host a skyrmion lattice, an appealing prospect for future integration into oxide electronic devices 2. With this in mind, there is a clear need for high quality SrFeO3 thin films, typically a challenge due to an unfavorable iron oxidation state and materials degradation 3. We synthesize and characterize SrFeO3 thin films grown by pulsed laser deposition, addressing these challenges by varying growth conditions and encapsulating layers.



1. Ishiwata, S. et al. Versatile helimagnetic phases under magnetic fields in cubic perovskite SrFeO3. Phys. Rev. B 84, 1–5 (2011).

2. Ishiwata, S. et al. Emergent topological spin structures in the centrosymmetric cubic perovskite SrFeO3. Phys. Rev. B 101, 134406 (2020).

3. Wang, L. et al. Time- and strain-dependent nanoscale structural degradation in phase change epitaxial strontium ferrite films. npj Mater. Degrad. 4, 3–8 (2020).

*Funding acknowledgements:Swiss National Science Foundation Postdoc.Mobility P400P2_199297US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract number DE-AC02-76SF00515Gordon and Betty Moore Foundation’s Emergent Phenomena in Quantum Systems Initiative through grant number GBMF9072

Presenters

  • Jennifer Fowlie

    • Stanford University
    • Stanford University, SLAC National Accelerator Laboratory

Authors

  • Jennifer Fowlie

    • Stanford University
    • Stanford University, SLAC National Accelerator Laboratory
  • Woojin Kim

    • Stanford University
    • Stanford Institute for Materials and Energy Sciences
  • Harold Hwang

    • Stanford Univ
    • Stanford University