Re-investigation of Moment Direction in Kitaev Material: α-RuCl3

ORAL

Abstract

α-RuCl3 has been attaining attention due to its possible realization of quantum spin liquid. While a signature of quantum spin liquid was observed in this material [1], the result has been controversial due to discrepancies between samples [2,3]. Here, we report X-ray diffraction and resonant elastic X-ray scattering (REXS) studies on α-RuCl3 crystals with distinct magnetic transition temperature of TN = 7.2K and 6.5K. We find the sample with TN = 6.5K exhibits a high degree of twinning, whereas the TN = 7.2K sample primarily comprises a single domain of R3. We find that both samples had identical magnetic structure with magnetic moments pointing away from the honeycomb plane by α=31± 2. We argue that the identical moment directions across these samples suggest that intralayer magnetic Hamiltonian remains mostly unchanged regardless of TN. Moreover, we propose that the observed sample-dependent variations in magnetic transition temperature within α-RuCl3 can be attributed to the interlayer interaction.

* Work at the University of Toronto was supported by the Natural Science and Engineering Research Council (NSERC) of Canada, Canadian Foundation for Innovation, and Ontario Research Fund. Diffraction work is based on research conducted at the Center for High-Energy X-ray Sciences (CHEXS), which is supported by the National Science Foundation. This research used resources at 6-ID beamline of the National Synchrotron Light Source II (NSLS-II), a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Brookhaven National Laboratory.

Publication: [1] Y. Kasahara et al., Nature 559, 227 (2018)
[2] P. Czajka et al., Nat. Phys. 17, 915 (2021)
[3] E. Lefrancois et al., Phys. Rev. X 12 021025 (2022)

Presenters

  • Subin Kim

    Univ of Toronto

Authors

  • Subin Kim

    Univ of Toronto

  • Ezekiel Horsley

    Univ of Toronto

  • Young-June Kim

    Univ of Toronto

  • Christie Nelson

    Brookhaven National Laboratory

  • Jacob Ruff

    Cornell University