Low-energy charge dynamics of infinite-layer nickelates: evidence for d-wave superconductivity

ORAL

Abstract

The discovery of superconductivity in infinite-layer nickelates establishes a new category of unconventional superconductors that shares structural and electronic similarities with cuprates. Despite the exciting advances, the key issues of the superconducting pairing symmetry, gap amplitude, superconducting fluctuation and collective modes remain elusive. In this talk, I will show how we utilize static and ultrafast terahertz spectroscopy to address these outstanding problems. We demonstrate that the equilibrium terahertz conductivity and nonequilibrium terahertz responses of an optimally Sr-doped nickelate film (Tc = 17 K) are in line with the electrodynamics of d-wave superconductivity in the dirty limit. The gap-to-Tc ratio is extracted to be 3.4, which indicates the superconductivity falls in the weak-coupling regime. In addition, we observed significant superconducting fluctuation near Tc. These results highlights a new d-wave system which closely resembles the electron-doped cuprates, expanding the family of unconventional superconductivity in oxides. Finally, we will present evidence for highly damped Higgs mode in infinite-layer nickelates.

* This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering (Ames National Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358). Work at SIMES was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC02-76SF00515 and the Gordon and Betty Moore Foundation’s Emergent Phenomena in Quantum Systems Initiative.

Publication: arXiv:2310.02586 (2023)
arXiv:2310.02589 (2023)

Presenters

  • Bing Cheng

    Ames National Laboratory

Authors

  • Bing Cheng

    Ames National Laboratory

  • Di Cheng

    Iowa State University

  • Kyuho Lee

    Stanford University

  • Liang Luo

    Ames National Laboratory, Ames Laboratory

  • Zhuoyu Chen

    Stanford University

  • Yonghun Lee

    Stanford University

  • Bai Yang Wang

    Stanford University

  • Martin Mootz

    Iowa State University, Ames National Laboratory

  • Chuankun Huang

    Iowa State University

  • Ilias Perakis

    University of Alabama at Birmingham

  • Zhi-Xun Shen

    Stanford University, stanford university

  • Harold Hwang

    Stanford University

  • JIGANG Wang

    Iowa State University