Harnessing chemical reactions for quantum science

ORAL

Abstract

Chemical reactions through collisions are often seen as violent processes, where chemical bonds break and form. Can quantum coherence be preserved throughout the entire reaction? Can chemical reactions be harnessed to produce entangled product pairs as quantum resources? Here, we investigate these questions by studying a ‘model’ gas-phase reaction 2KRb → K2 + Rb2 at ultracold temperatures, focusing on the nuclear spin degrees of freedom. In particular, we prepare the initial nuclear spins in KRb in an entangled state and characterize the preserved coherence in the nuclear spin wavefunction after the reaction by measuring the product state distribution. We find that the coherence in reactants is almost fully preserved, suggesting that entanglement can be prepared within the reactants, followed by a chemical reaction that produces separate, entangled molecules.

* This work is funded by NSF-EAGER through Grant~CHE-2332539, the Gordon and Betty Moore Foundation through GBMF11558, and the David and Lucile Packard Foundation.

Publication: arXiv: 2310.07620

Presenters

  • Yi-Xiang Liu

    Harvard University

Authors

  • Yi-Xiang Liu

    Harvard University

  • Lingbang Zhu

    Harvard University

  • Jeshurun Luke

    Harvard University

  • Arfor Houwman

    Universität Innsbruck

  • Mark Babin

    Harvard University

  • Ming-Guang Hu

    QuEra Computing

  • Kang-Kuen Ni

    Harvard University