Anomalous Purcell decay of strongly driven and disordered emitters coupled to a cavity (Part 2): Theory

ORAL

Abstract

Arrays of quantum emitters interacting with cavities offer insights into the interplay of many-body quantum dynamics and collective emission. Motivated by recent experimental progress, we study a disordered ensemble of spins realized with Er3+ ions coupled to a laser-driven nanophotonic cavity. The light emission from the cavity following an initial excitation pulse exhibits a non-trivial reduction at cavity resonance, leading to a double-peak structure reminiscent of vacuum Rabi splitting, but persistent at long times and dependent on initial excitation power. These observations suggest a non-trivial modification of conventional Purcell decay physics in this strongly driven, strongly disordered system. We theoretically characterize the dynamics of the light field and collective spin observables with a variety of techniques, including semi-classical approaches and Holstein-Primakoff mappings. The role of collective effects and spin-spin interactions mediated by the cavity is identified and characterized. Comparisons of the theory to the experimental data are made

* The authors acknowledge the Q-NEXT Quantum Center, a U.S. Department of Energy, Office of Science, National Quantum Information Science Research Center, under Award Number DE-FOA-0002253 for support.

Publication: M. T. Solomon et al. "Anomalous Purcell decay of strongly driven inhomogeneous emitters coupled to a cavity." arXiv, DOI: 10.48550/arXiv.2309.16641 (2023)

Presenters

  • Mikhail Mamaev

    University of Chicago

Authors

  • Mikhail Mamaev

    University of Chicago

  • Martin Koppenhoefer

    University of Chicago

  • Michael T Solomon

    University of Chicago

  • Cheng Ji

    University of Chicago / Argonne National Lab, University of Chicago

  • Gregory Grant

    University of Chicago / Argonne National Lab, University of Chicago

  • Ignas Masiulionis

    University of Chicago / Argonne National Lab, University of Chicago/Argonne National Laboratory, University of Chicago

  • Sean E Sullivan

    Argonne National Laboratory

  • F. Joseph F Heremans

    Argonne National Laboratory, Argonne National Lab, Argonne, University of Chicago

  • Supratik Guha

    Argonne National Laboratory, University of Chicago/Argonne National Laboratory

  • David D Awschalom

    University of Chicago

  • Alan M Dibos

    Argonne National Laboratory, Argonne National Lab

  • Aashish A Clerk

    University of Chicago