Title: Spectroscopic evidence for topological band structure in FeTe0.55Se0.45

ORAL

Abstract

FeTe0.55Se0.45(FTS) occupies a special spot in modern condensed matter physics at the intersections of electron correlation, topology, and unconventional superconductivity. The bulk electronic structure of FTS is predicted to be topologically nontrivial thanks to the band inversion. between the dxz and pz bands along Γ-Z. This in turn would give rise to a Dirac surface state (DSS) hosting topological superconductivity below the bulk superconducting temperature. However, whether this prediction is indeed realized in FTS remains controversial in recent angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling spectroscopy (STS) studies. In ARPES experiments, a Dirac-cone-like feature has been identified, yet only at certain out-of-plane momenta (kz), leading to speculations that it might originate from a bulk band instead of the DSS. Moreover, the measured band structure differs significantly from the density functional theory (DFT) predictions, with no direct observations of either the pz band or the bulk band inversion. Here we resolve this debate through a comprehensive ARPES investigation. We first observe a persistent DSS independent of kz. Then, by comparing FTS with FeSe which has no band inversion along Γ-Z, we identify the spectral weight fingerprint of both the presence of the pz band and inversion between the dxz and pz bands. Our results highlight the impact of band renormalization and large spin-orbit coupling in FTS and make a strong case for the existence of topological band structure in this unconventional superconductor.

* Synchrotron ARPES measurements were performed at Beamline 5-2 and 5-4, Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory. The works at Stanford University and SLAC are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-76SF00515. Support for FTS crystal growth and characterization at Penn State is provided by the National Science Foundation through the Penn State 2D Crystal Consortium-Materials Innovation Platform (2DCC-MIP) under NSF Cooperative Agreement DMR-2039351.

Publication: http://arxiv.org/abs/2307.03861

Presenters

  • Yingfei Li

    Department of Applied Physics, Stanford University

Authors

  • Yingfei Li

    Department of Applied Physics, Stanford University