Oral: Large anomalous Hall effect, topological Hall effect, skyrmions, and disorder observed in Fe3GaTe2

ORAL

Abstract

Fex(Ge:Ga)Te2 compounds captivate with their topological electronic and magnetic structure, inherent disorder, and high magnetic transition temperatures. Here, we present findings on the Fe3GaTe2 single crystal, which is the newest member of the Fex(Ge:Ga)Te2 compounds. Magnetization data pinpoints a ferromagnetic transition near 360 K. At room temperature, we observed a substantial anomalous Hall resistivity ~ 20 μΩcm and evidence of the topological Hall effect. The Lorentz transmission tunneling microscope unveiled prevalent stripe and skyrmion domain structures above room temperature, hinting at the topological spin texture as an origin of the topological Hall effect. Remarkably, single crystal X-ray diffraction unveiled significant disorder due to the migration of Fe atoms from the intralayer to interlayer positions. We found that annealing at low temperatures effectively mitigates this disorder, leading to decreased resistivity and increased anomalous Hall conductivity. By adjusting the disorder through annealing and analyzing extensive experimental data across a wide range of temperatures and magnetic fields, we delve into the intricate relationship between structural disorder, magnetic structure, and electron transport properties.

* This work is supported by the Department of Energy, Basic Energy Sciences program, grant # DE-SC0002613, and the National Research Foundation of Korea (NRF-2022H1D3A3A01077468).

Presenters

  • Sang-Eon Lee

    National High Magnetic Field Laboratory

Authors

  • Sang-Eon Lee

    National High Magnetic Field Laboratory

  • Vadym Kulichenko

    National High Magnetic Field Laboratory

  • Alex Moon

    National High Magnetic Field Laboratory

  • Lingrui Mei

    National High Magnetic Field Laboratory

  • Kice Brown

    Baylor University

  • Julia Y Chan

    Baylor University

  • Yue Li

    Argonne National Laboratory

  • Gregory T McCandless

    Baylor University

  • Charudatta M Phatak

    Argonne National Laboratory, Argonne National Lab

  • Luis Balicas

    National High Magnetic Field Laboratory, Florida State University, National High Magnetic Field Laboratory