Emergent spin-gapped magnetization plateaus in a spin-1/2 perfect kagome antiferromagnet

ORAL

Abstract

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the presence or absence of the 1/9 magnetization plateau, where exotic quantum states, including topological ones, are expected to emerge. Here we report the magnetization of a recently discovered kagome QSL candidate YCu3(OH)6.5Br2.5 up to 57 T. Above 50 T, a clear magnetization plateau at 1/3 of the saturation moment of Cu2+ ions is observed, supporting that this material provides an ideal platform for the kagome Heisenberg antiferromagnet. Remarkably, we found another magnetization plateau around 20 T, which is attributed to the 1/9 plateau. The temperature dependence of this plateau reveals the distinct spin gap, whose magnitude estimated by the plateau width is approximately 10% of the exchange interaction. The observation of 1/9 and 1/3 plateaus highlights the emergence of novel states in quantum spin systems.

* This work is supported by Grants-in-Aid for Scientific Research (KAKENHI) (Nos. 23K13060 and 23H00089) and on Innovative Areas ``Quantum Liquid Crystals'' (No. JP19H05824) from the Japan Society for the Promotion of Science, and JST CREST (JPMJCR19T5). The work in Wuhan was supported by the National Natural Science Foundation of China (No. 12274153).

Publication: S. Suetsugu et al., arXiv:2310.10069 (2023).

Presenters

  • Shota Suetsugu

    Kyoto Univ, Kyoto University

Authors

  • Shota Suetsugu

    Kyoto Univ, Kyoto University

  • Tomoya Asaba

    Kyoto University

  • Yuichi Kasahara

    Kyoto University, Kyoto Univ

  • Yuhki Kohsaka

    Kyoto University, Kyoto Univ

  • Keisuke Totsuka

    Kyoto University

  • Boqiang Li

    Huazhong University of Science and Technology

  • Yuqiang Zhao

    Huazhong University of Science and Technology

  • Yuesheng Li

    Huazhong University of Science and Technology

  • Masashi Tokunaga

    The Institute for Solid-State Physics, University of Tokyo, The University of Tokyo, University of Tokyo, ISSP

  • Yuji Matsuda

    Kyoto Univ, Kyoto University