How nonlinearity distorts the evidence for photoinduced superconductivity

ORAL · Invited

Abstract

We have recently identified a fundamental flaw in the analysis of several influential results on photoinduced superconductivity in K3C60. We have also shown that similar measurements on other compounds suffer from the same problem. I will show how this systematic error distorts the existing evidence for both photoinduced superconductivity and Higgs-mediated terahertz amplification in K3C60. When we account for this error, we find that the experiments on K3C60 may be understood instead as a photoenhancement of its carrier mobility that saturates with fluence, with no need to appeal to a photoinduced phase transition to a superconducting state. I will describe how this error also distorts the evidence for photoinduced superconductivity in the normal state of cuprate superconductors and the charge-transfer salt BEDT-TTF. Finally, I will describe how recent work on K3C60 provides quantitative support for our analysis.

* J.S.D. acknowledges support from NSERC and CIFAR, and D.G.S. from an NSERC Alexander Graham Bell Canada Graduate Scholarship.

Publication: J. S. Dodge, L. Lopez, and D. G. Sahota, "Optical Saturation Produces Spurious Evidence for Photoinduced Superconductivity in K3C60", Phys. Rev. Lett. 130, 146002 (2023).

Presenters

  • J. Steven Dodge

    Simon Fraser University

Authors

  • J. Steven Dodge

    Simon Fraser University

  • Derek G Sahota

    Simon Fraser Univ

  • Leya Lopez

    Simon Fraser University