Universal sublinear resistivity in vanadium kagome materials hosting charge density waves

ORAL

Abstract

The recent discovery of a charge density (CDW) state in ScV6Sn6 at TCDW = 91 K offers new opportunities to understand the origins of electronic instabilities in topological kagome systems. By comparing to the isostructural non-CDW compound LuV6Sn6, we unravel interesting electrical transport properties in ScV6Sn6, above and below TCDW. We observed that by applying a magnetic field along the a axis, the temperature behavior of the longitudinal resistivity in ScV6Sn6 changes from metal-like to insulator-like above the CDW transition. We show that in the charge ordered state ScV6Sn6 follows the Fermi liquid behavior while above that, it transforms into a non-Fermi liquid phase in which the resistivity varies sublinearly over a broad temperature range. The sublinear resistivity, which scales by T3/5 is a common feature among other vanadium-containing kagome compounds exhibiting CDW states such as KV3Sb5, RbV3Sb5, and CsV3Sb5. By contrast, the non-Fermi liquid behavior does not occur in LuV6Sn6. We explain the T3/5 universal scaling behavior from the Coulomb scattering between Dirac electrons and Van Hove singularities; common features in the electronic structure of kagome materials. Finally, we show anomalous Hall-like behavior in ScV6Sn6 below TCDW, which is absent in the Lu compound. Comparing the transport properties of ScV6Sn6 and LuV6Sn6 is valuable to highlight the impacts of the unusual CDW in the Sc compound.

* SM, RPM, and DM supported by AFOSR MURI grant# FA9550-20-1-0322. WRM and HWSA suppported by the Gordon and Betty Moore Foundation's EPiQS, Grant GBMF9069 to DM. Theory work by YZ was supported from the start-up fund at the University of Tennessee. Theory at the Oak Ridge supprted by the US DoE, Office of Science, QSC (S-H K), and the Materials Sciences and Engineering Division (JWV and MY). The Oak Ridge Leadership Computing Facility at the ORNL, supported by the Office of Science of the U.S. DoE Contract No. DE-AC05-00OR22725 and the NERSC, a DOE Office of Science User Facility supported by the Office of Science of the US DoE contract No. DE-AC02-05CH11231 using NERSC award BES-ERCAP0024568. LL supported by NSF Award No.DMR-2004288 and DoE Award No. DE-SC0020184.

Publication: https://doi.org/10.48550/arXiv.2305.02393

Presenters

  • Shirin Mozaffari

    University of Tennessee, Knoxville

Authors

  • William R Meier

    University of Tennessee, Knoxville

  • Shirin Mozaffari

    University of Tennessee, Knoxville

  • Richa Madhogaria

    University of Tennessee, University of Tennessee, Knoxville

  • Nikolai Peshcherenko

    Max Planck Institute for Chemical Physics of Solids

  • Seoung-Hun Kang

    Oak Ridge National Laboratory, Oak Ridge National Lab

  • John W Villanova

    Oak Ridge National Laboratory

  • Hasitha W Arachchige

    University of Tennessee, Knoxville

  • Guoxin Zheng

    University of Michigan

  • Yuan Zhu

    University of Michigan

  • Kuan-Wen Chen

    University of Michigan

  • Kaila G Jenkins

    University of Michigan

  • Dechen Zhang

    University of Michigan

  • Aaron L Chan

    University of Michigan, Ann Arbor

  • Lu Li

    University of Michigan

  • Mina Yoon

    Oak Ridge National Laboratory, Oak Ridge National Lab

  • Yang Zhang

    University of Tennessee, Knoxville, University of Tennessee, IAMM HQ, University of Tennessee Knoxville

  • David Mandrus

    University of Tennessee