Magnetic ground state of the pyrochlore iridate Ho2Ir2O7

ORAL

Abstract

Rare-earth pyrochlore iridates R2Ir2O7 (e.g., R = Y, rare-earth elements) are an exciting class of quantum materials that exhibit emergent electronic and magnetic phenomena. A little-explored member of the family, Ho2Ir2O7, has been reported as a spin-ice iridate; however, the presence of two distinct magnetic sublattices on Ho3+ (4f-electrons) and Ir4+ (5d-electrons) has opened intriguing questions about each sublattice contribution to the overall electronic and magnetic properties of this pyrochlore iridate. In this talk, we will present our recent results on the first successful synthesis of high-quality large-size (111)-oriented Ho2Ir2O7 thin films and mapping the magnetic ordering of the Ir sublattice. Our results reveal the intriguing effects of the large Ho moments on the Ir ordering.

* J. C. acknowledges the support by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0022160. J. Z. acknowledges the support by the National Science Foundation through the Center for Dynamics and Control of Materials: an NSF MRSEC under Cooperative Agreement No. DMR-1720595 and DMR-2308817.

Presenters

  • Colby Stoddard

    Rutgers New Brunswick

Authors

  • Colby Stoddard

    Rutgers New Brunswick

  • Michael Terilli

    Rutgers University

  • Tsung-Chi Wu

    Rutgers University, New Brunswick

  • Mikhail Kareev

    Rutgers University, New Brunswick

  • Jak Chakhalian

    Rutgers University

  • Yue Cao

    Argonne National Laboratory

  • Hao Zheng

    Argonne National Laboratory

  • Christie Nelson

    Brookhaven National Laboratory

  • Hongze Li

    University of Texas at Austin

  • Jianshi Zhou

    University of Texas at Austin