Unconventional Signatures of a Quantum Griffiths Phase in the Vicinity of a Quenched Nematic Quantum Critical Point

ORAL · Invited

Abstract

Upon suppression of a continuous electronic phase transition towards 0K, for example through hydrostatic pressure as an external tuning parameter, a quantum critical point (QCP) occurs in many different material classes. These points constitute a fascinating research area as the diverging quantum fluctuations and electronic correlations could be linked to many unconventional and exciting quantum phases, including the emergence of high-Tc superconductivity. Nevertheless, even more exotic phase may be expected if the symmetry of the electronic order parameter allows for a bilinear coupling to the structural degrees of freedom. The electronic nematic order, ubiquitous in the iron-based superconductors, is one such candidate, where long-range interactions can be mediated through the lattices shear modes.

In this talk, we will first review the unique nature of the isolated nematic QCP in FeSe0.89S0.11 under hydrostatic pressure, in the absence of any competing electronic order. At this point, the nematoelastic coupling quenches the quantum critical fluctuations and hence, superconductivity is weakened instead of enhanced. We will then demonstrate that the magnetoresistivity close to the QCP obeys a scaling relation over two decades in temperature with diverging critical exponents at low temperatures. Such divergences are in a stark contrast to the usual ansatz using fixed exponents and the notion of universality classes. We will discuss our findings in the context of an unusual quantum Griffiths phase, emerging from disconnected static and dynamic quantum fluctuations. Moreover, the coupling between the electronic and phononic modes and a possible topological change of the Fermi surface lead to the emergence of an atypical non-zero energy scale at the QCP, consistent with the observation of finite electronic correlations.

* We acknowledge funding from the EPSRC (EP/I004475/1, EP/I017836/1, EP/M020517/1, EP/N01085X/1), the NSF (DMR-1157490, DMR-1828489), the State of Florida, and the University of Oxford John Fell Fund

Publication: * P. Reiss, D.E. Graf, A.A. Haghighirad, W. Knafo, L. Drigo, M. Bristow, A.J. Schofield, A.I. Coldea: Quenched nematic criticality and two superconducting domes in an iron-based superconductor. Nature Physics 16, 89-94 (2020). http://www.nature.com/articles/s41567-019-0694-2
* P. Reiss, D.E. Graf, A.A. Haghighirad, T. Vojta, A.I. Coldea: Signatures of a Quantum Griffiths Phase Close to an Electronic Nematic Quantum Phase Transition. Physical Review Letters 127, 246402 (2021). https://link.aps.org/doi/10.1103/PhysRevLett.127.246402
* P. Reiss, A. McCollam, Z. Zajicek, A.A. Haghighirad, A.I. Coldea: Collapse of Metallicity and High-Tc Superconductivity in the High-Pressure phase of FeSe0.89S0.11. arXiv:2212.06824

Presenters

  • Pascal Reiss

    Max Planck Institute for Solid State Research

Authors

  • Pascal Reiss

    Max Planck Institute for Solid State Research

  • David E Graf

    Florida State University, National High Magnetic Fields Laboratory, Florida State University, National High Magnetic Field Laboratory, Florida State University

  • Amir A Haghighirad

    Karlsruhe Institute of Technology, IQMT, Karlsruhe Institute of Technology

  • Matt Bristow

    University of Oxford

  • Zachary Zajicek

    University of Oxford

  • William Knafo

    LNCMI

  • Andrew Schofield

    Lancaster University

  • Thomas Vojta

    Missouri University of Science & Technol

  • Amalia I Coldea

    University of Oxford