Imaging the many-body wavefunctions in magic-angle graphene

ORAL

Abstract

Magic-angle twisted bilayer graphene (MATBG) hosts a set of flat electronic bands that produce a wide variety of correlated ground states including superconductors, correlated insulators, and magnetic topological phases. Our understanding of these phases has thus far been hampered by the lack of microscopic, atomic-scale information on them. In this talk, I will discuss how we use high-resolution scanning tunneling microscopy (STM) measurements to study the wavefunctions of these correlated phases. STM images reveal distinct symmetry-breaking patterns with a sqrt(3) x sqrt(3) superperiodicity on the graphene atomic lattice. To understand these patterns, we develop a symmetry-based analysis to visualize the images in terms of a set of complex-valued order parameters. At the correlated insulators at fillings ±2 electrons per moiré unit cell, comparison with theoretical candidates reveals a close match with the proposed incommensurate Kekulé spiral order in samples with typical values of interlayer strain, while in ultralow-strain samples, our data have local symmetries resembling the time-reversal symmetric intervalley coherent phase. These symmetry-based techniques can be further applied to other phases in MATBG, graphene systems, and potentially other material systems.

* This work was primarily supported by the Gordon and Betty Moore Foundation's EPiQS initiative grants GBMF9469 and DOE-BES grant DE-FG02-07ER46419 to A.Y. Other support for the experimental work was provided by NSF-MRSEC through the Princeton Center for Complex Materials NSF-DMR- 2011750, NSF-DMR-1904442, ARO MURI (W911NF-21-2-0147) and ONR N00012-21-1-2592. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan, grant JPMXP0112101001, JSPS KAKENHI grants 19H05790 and JP20H00354.

Publication: Nuckolls, K.P., Lee, R.L., Oh, M. et al. Quantum textures of the many-body wavefunctions in magic-angle graphene. Nature 620, 525–532 (2023). https://doi.org/10.1038/s41586-023-06226-x

Presenters

  • Ryan L Lee

    Princeton University

Authors

  • Ryan L Lee

    Princeton University

  • Kevin P Nuckolls

    Massachusetts Institute of Technology

  • Myungchul Oh

    Princeton University, Pohang University of Science and Technology

  • Dillon Wong

    Princeton University

  • Tomohiro Soejima

    Harvard University; IBM Quantum, Almaden Research Center, Harvard University

  • Jung Pyo Hong

    Princeton University

  • Dumitru Calugaru

    Princeton University

  • Jonah Herzog-Arbeitman

    Princeton University

  • Andrei B Bernevig

    Princeton University

  • Kenji Watanabe

    National Institute for Materials Science, NIMS, Research Center for Electronic and Optical Materials, National Institute for Materials Science, Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science

  • Takashi Taniguchi

    Kyoto Univ, National Institute for Materials Science, Research Center for Materials Nanoarchitectonics, Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, National Institute for Materials Sciences, NIMS, International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, National Institute for Material Science, International Center for Materials Nanoarchitectonics, NIMS, Japan, International Center for Materials Nanoarchitectonics, Tsukuba, National Institue for Materials Science, Kyoto University, National Institute of Materials Science, International Center for Materials Nanoarchitectonics and National Institute for Materials Science

  • Nicolas Regnault

    Princeton University

  • Michael P Zaletel

    University of California, Berkeley, University of Berkerley, UC Berkeley

  • Ali Yazdani

    Princeton University