Pulsed magnetic field studies of topological magnetic kagome compounds

ORAL

Abstract

Magnetic Weyl semimetals provide an interesting opportunity to study the interplay between local spin texture, band topology and correlations. The rare earth 166 kagome materials are a prime example, which exhibit complex magnetic orders driven by competing interactions and anisotropies, as well as an electronic structure that embodies both flat band and linear (Dirac) band crossings. Specifically, this includes ErMn6Sn6 which crystallizes in a hexagonal space group P6/mmm (No. 191). The recent neutron diffraction data shows that ErMn6Sn6 exhibits a first order transition from a planar-ferrimagnetic to distorted triple-spiral magnetic order at T = 92 K and the theoretical calculations using the mean-field theory predict a very rich magnetic phase diagram of ErMn6Sn6 [1]. We present the experimental measurements of magnetization in pulsed magnetic field with H//a, H//b and H//c. The rich variety of magnetic phases gives us opportunity to study the behavior of Dirac fermions with control of the spin orientations tuned by the magnetic field. High field magnetoresistivity and Hall effect measurement helped us to identify novel magnetic and topological phases and probe Fermi surface topology via quantum oscillations. This combination of experiments reveals the possibility of tuning topological properties in ErMn6Sn6 via the application of strong magnetic fields.

[1] Riberolles, S. X. M, et al. arXiv preprint arXiv:2306.13206 (2023).

* The work was performed at the National High Magnetic Field Laboratory (NHMFL), which is supported by National Science Foundation Cooperative Agreement No. DMR-2128556 and the Department of Energy (DOE). This research is supported by the Center for the Advancement of Topological Semimetals (CATS), an Energy Frontier Research Center funded by the USDOE Office of Science, Office of Basic Energy Sciences, through the Ames Laboratory. Ames Laboratory is operated for the USDOE by Iowa State University under Contract No. DE-AC02-07CH11358.

Presenters

  • Joanna Blawat

    NHMFL, Los Alamos National Laboratory, Los Alamos National Laboratory

Authors

  • Joanna Blawat

    NHMFL, Los Alamos National Laboratory, Los Alamos National Laboratory

  • Tyler J Slade

    Ames National Lab, Ames National Laboratory

  • John Singleton

    National High Magnetic Field Laboratory

  • Benjamin G Ueland

    Ames National Laboratory/Iowa State University, Ames National Laboratory

  • Paul C Canfield

    Iowa State University, Ames National Laboratory/Iowa State University

  • Robert J McQueeney

    Ames National Laboratory/Iowa State University, Iowa State University, Ames National Laboratory and Iowa State University

  • Ross D McDonald

    Los Alamos National Laboratory