Dark-field x-ray microscopy with structured illumination

ORAL · Invited

Abstract

We propose a structured illumination technique for dark-field x-ray microscopy, enabling real-time, high-resolution, and bulk-sensitive observation of quantum solids. Unlike traditional tomography, our method projects a scanning x-ray silhouette, generated through a micro coded aperture, onto materials under a Bragg condition. This eliminates the need for sample rotation or rastering, ensuring a highly stable imaging process. This lens-based full-field x-ray diffraction method offers a range of contrast mechanisms, allowing for the observation of various phenomena in quantum materials. We present the concept of the microscope along with its imaging methods, and validate our findings with experimental data on nematic order obtained from a synchrotron undulator beamline.

* This research used resources of the Advanced Photon Source and the Center for Nanoscale Materials, U.S. Department of Energy (DOE) Office of Science User Facilities and is based on work supported by Laboratory Directed Research and Development (LDRD) funding from Argonne National Laboratory, provided by the Director, Office of Science, of the U.S. DOE under Contract No. DE-AC02-06CH11357. We thank the Karlsruhe Nano Micro Facility (KNMF) for the fabrication of the polymer X-ray optics.

Presenters

  • Doga Gursoy

    Argonne National Laboratory

Authors

  • Doga Gursoy

    Argonne National Laboratory

  • Kaan A Yay

    Stanford University

  • Elliot Kisiel

    University of California, San Diego, University of California, Davis

  • Michael Wojcik

    Argonne National Laboratory

  • Dina Sheyfer

    Argonne National Laboratory

  • Matthew J Highland

    Argonne National Laboratory

  • Ian R Fisher

    Stanford Univ, Stanford University

  • Stephan O Hruszkewycz

    Argonne National Laboratory

  • Zahir Islam

    Argonne National Laboratory