Role of dimensionality in CeIn3 nanowires

ORAL

Abstract

Quantum materials are remarkably complex systems where new emergent phenomena are likely to arise. In particular, low-dimensional strongly correlated materials provide an ideal platform for experimental discoveries. In this work, we have studied the routes for synthesizing intermetallic nanowires of CeIn3 by the Metallic-Flux Nanonucleation (MFNN) method [1] and the effects of dimensionality via structural and magnetic measurements. The study of emergent phenomena in one-dimensional systems was previously reported in different systems grown using MFNN [2]–[5].

We successfully obtain nanowires (d =170 ± 5 nm) and single crystals, which we investigate by means of Energy Dispersive Spectroscopy (EDS), magnetic susceptibility, and heat capacity. Semiquantitative EDS analysis indicates a ratio of 1:3.1(1) of Ce:In in the nanowires, which is consistent with the desired stoichiometry. Magnetic susceptibility and specific heat data showed a suppression of the antiferromagnetic transition from the bulk TN ~ 10 K. Our findings suggest a strong dimensionality effect on magnetic properties. To obtain a better understanding of this effect, electrical transport measurements of isolated nanowires will be required.

* Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering.This work was supported by the FAPESP (grants No 2020/10580-8 and 22/16823-5)

Publication: [1] K.R. Pirota, et al., P BR patent 10 2014 019794 0, 2014
[2] K. O. Moura et al., Sci. Rep., vol. 6, no. June, pp. 1–9, 2016
[3] K. O. Moura et al., Sci. Rep., vol. 7, no. 1, pp. 3–9, 2017
[4] A. dos S. E. d. Cruz et al., Nanoscale Adv., vol. 3, no. 11, pp. 3251–3259, 2021
[5] P. F. S. Rosa et al., Solid State Commun., vol. 191, pp. 14–18, 2014

Presenters

  • Maria Helena Carvalho da Costa

    Los Alamos National Laboratory

Authors

  • Maria Helena Carvalho da Costa

    Los Alamos National Laboratory

  • Henrique Pizzi

    UNICAMP

  • Gabriel Silva Freitas

    UNICAMP

  • A. Caffer

    UNICAMP

  • K. Pirota

    UNICAMP

  • Priscila Rosa

    Los Alamos National Laboratory

  • P. G. Pagliuso

    UNICAMP