New Color Centers in Diamond for Quantum Applications

ORAL

Abstract

Color centers in diamond are promising platforms for quantum communication and quantum sensing applications. All the defects in diamond reported so far emit photons in the visible to near-infrared region, which experience high losses in fiber optics and scattering media such as biological samples. Furthermore, no color centers observed thus far exhibit coherence times comparable to nitrogen vacancies at elevated temperatures. Here, we report the experimental observation of two new color centers in diamond that emit in the telecom band. The first color center emits in the telecom O-band [1]. From absorption, photoluminescence, and transient absorption spectroscopy, we identify a zero-phonon line at 1221 nm with phonon replicas separated by 42 meV and an excited state lifetime of ~270 ps. The second is substitutional Er3+ incorporated in diamond, which emits in the telecom C-band. Finally, we deploy our spectroscopy and materials characterization pipeline to investigate other new defects in diamond as potential candidates for quantum sensing by characterizing spin dynamics using pulsed electron spin resonance.



[1] S. Mukherjee et al., Nano Lett. 2023, 23, 7, 2557–2562.

Publication: S. Mukherjee et al., Nano Lett. 2023, 23, 7, 2557–2562.

Presenters

  • Sounak Mukherjee

    Princeton University

Authors

  • Sounak Mukherjee

    Princeton University

  • Zihuai Zhang

    University of California, Berkeley and Lawrence Berkeley National Laboratory, Princeton University, University of California, Berkeley, University of California, Berkeley; Lawrence Berkeley National Laboratory

  • Sean Karg

    Princeton University

  • Arunava Das

    Princeton University

  • Daniel G Oblinsky

    Princeton University

  • Sebastian P Horvath

    Princeton University

  • Mayer M Feldman

    Princeton University

  • Mitchell O de Vries

    RMIT University

  • Brett C Johnson

    RMIT University

  • Brant C Gibson

    RMIT University

  • Edwin L H Mayes

    RMIT University

  • Andrew M Edmonds

    Element Six

  • Nicola Palmer

    Element Six

  • Matthew L Markham

    Element Six

  • Ádám Gali

    Wigner Research Centre for Physics

  • Gergő Thiering

    Wigner Research Centre for Physics, Wigner Research Centre

  • Adam Dalis

    Hyperion Materials & Technologies

  • Timothy Dumm

    Hyperion Materials & Technologies

  • Gregory D Scholes

    Princeton University

  • Alastair Stacey

    RMIT University, School of Science, RMIT University, Melbourne, Victoria 3000, Australia

  • Philipp Reineck

    RMIT University

  • Jeff D Thompson

    Princeton University

  • Stephen A Lyon

    Princeton, EeroQ Corp., Princeton University, EeroQ Corp, Princeton University, EeroQ Corp., Princeton University

  • Nathalie P de Leon

    Princeton University