Orbital Rashba effects and light-induced Orbital Current in Teraherz Emission Experiments.

ORAL · Invited

Abstract

Orbitronics is based on the use of orbital currents as information carriers. These may be generated by the application of an electric field, and inversely, by reciprocity, they could be converted back to charge or even spin currents. In this presentation, I will start my presentation by describing experiments showing the strong enhancement of the current-induced torques on the Co layer of a Pt/Co bilayer by the addition of an Al layer on Co (Al protected from oxidation). The enhancement is predominant for the FL torque, up to factor of 9. The interpretation [2] comes from ab-initio calculations showing large Co orbital moments in the interfacial Co layer with a helical texture similar to the spin texture on the surface of topological insulators. The calculation of the resulting torques leads to a good agreement between the calculated and enhanced experimental torques.

In a second part, we will demonstrate that orbital currents can also be generated by femtosecond light pulses and optical absorption on thin Ni films. In multilayers associating Ni with oxides and nonmagnetic metals such as Cu, we detect the generated orbital currents by their conversion into charge currents varying in time in the subpicosecond scale and thus resulting in a terahertz emission as provided by oscillating dipoles. We show that the orbital currents extraordinarily predominate the light-induced spin currents in Ni-based systems, whereas, unlike, only spin currents can be detected with CoFeB-based similar systems and heterostructures. In addition, the analysis of the time delays of the terahertz pulses leads to relevant information on the group velocity and subsequent propagation of orbital carriers. Our finding of light-induced orbital currents and our observation of their conversion into charge currents opens new avenues in orbitronics, including the development of novel type of orbitronic terahertz devices

* National Key Research and Development Program of China (No. 2022YFB4400200)National Natural Science Foundation of China (No. 92164206,62105011, 11904016, 52261145694 and 52121001)Beihang Hefei Innovation Research Institute Project (BHKX-19-01, BHKX-19-02)ANR program ORION through Grant No. ANR-20-CE30-0022-02

Publication: S. Krishnia et al., Nano Lett. 2023, 23, 15, 6785–6791

Presenters

  • Henri Jaffres

    Unite Mixte de Physique CNRS/Thales, Unité Mixte de Physique CNRS-Thales

Authors

  • Henri Jaffres

    Unite Mixte de Physique CNRS/Thales, Unité Mixte de Physique CNRS-Thales

  • Yong Xu

    MIIT Key Laboratory of Spintronics, School of Integrated Circuit Science and Engineering, Beihang University

  • Albert Fert

    CNRS/THALES

  • Weisheng ZHAO

    BeiHang University

  • Vincent Cros

    UMPHY CNRS-Thales

  • Sachin Krishnia

    UMPHY CNRS-Thales

  • Nicolas Sebe

    UMPHY CNRS-Thales

  • Nicolas Reyren

    Unit?© Mixte de Physique, CNRS, Thales,

  • Jean-Marie George

    UMPHY CNRS-Thales, Université Paris-Saclay