Quantum-critical scaling in the Mn-based kagome metal Sc3Mn3Al7Si5

ORAL

Abstract

Kagome lattices can host a variety of exotic ground states, including quantum spin liquids and correlated phases associated with dispersionless flat energy bands. The Mn-based kagome metal Sc3Mn3Al7Si5 crystalizes a hexagonal structure in which Mn ions form a kagome network, and shows unusual behavior in transport and thermodynamic properties [1]. Interestingly, a recent study, supported by theoretical calculations, has suggested the presence of orbital-selective flat-band-induced ferromagnetic fluctuations [2]. To elucidate the flat-band-induced ferromagnetic instability, we synthesized single crystals of Sc3Mn3Al7Si5 and measured charge transport and heat capacity at very low temperatures. We observe no anomaly associated with long-range order in resistivity down to 15 mK and a logarithmic divergence in low-temperature heat capacity. The logarithmic divergence in heat capacity is strongly suppressed by magnetic fields, suggesting a crossover from non-Fermi-liquid to Fermi-liquid behavior, often observed in quantum critical metals. This anomalous crossover in heat capacity is well described by quantum-critical scaling. We will discuss the relationship between the quantum criticality and orbital-selective flat bands in the kagome metal Sc3Mn3Al7Si5.

* C.D. and Y.N. were supported by an NSF Career DMR-1944975. The National High Magnetic Field Laboratory is supported by the National Science Foundation through NSF/DMR-1644779 and the State of Florida.

Publication: [1] H. He et al., Inorganic Chemistry 53, 17 (2014).
[2] S. Samanta et al., arXiv:2304.04928.

Presenters

  • Yasuyuki Nakajima

    University of Central Florida

Authors

  • Yasuyuki Nakajima

    University of Central Florida

  • Charuni Dissanayake

    University of Central Florida

  • Kapila Kumarasinghe

    University of Central Florida

  • Mark Tomlinson

    University of Central Florida

  • Eun Sang Choi

    National High Magnetic Field Laboratory, National High Magnetic Field Lab, Tallahassee, Florida, NHMFL, MagLab, Florida State University, National High Magnetic Field Laboratory, Florida State University