All-optically injected photocurrents in topologically insulating Bi2Se3

ORAL

Abstract

Nonlinear optics techniques have been employed to provide an all-optical method to generate and control photocurrents in semiconductors. Inevitably arises the challenge of distinguishing various processes that contribute to the photocurrent. This talk reports the generation of shift and injection currents simultaneously in topologically insulating bismuth selenide (Bi2Se3) thin films. A near-infrared pump and its phase-related frequency-doubled counterpart excite the currents, which are detected through their terahertz radiation. The properties of the photocurrents, such as their magnitude and direction relative to the polarization of the incident fields, are compared to theoretical predictions based on the symmetries of the crystal lattice, allowing the different photocurrents to be isolated. This work thus presents a comprehensive all-optical method for analyzing the optoelectronic properties of topological insulators.

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Authors

  • Derek Bas

    West Virginia University

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division

  • Scott Cushing

    National Radio Astronomy Observatory, Jodrell Bank Centre for Astrophysics, New York University Abu Dhabi, Naval Research Laboratory, CSIRO Astronomy and Space Sciences, George Mason University, ASTRON, NASA Goddard Space Flight Center, University of Wisconsin-Milwaukee,, Station de radioastronomie de Nancay, Columbia Astrophysics Laboratory, Max-Planck-Institut fur Physik, West Virginia Univ, West Virginia University, Lehigh University, Fraunhofer Institute for Physical Measurement Techniques, Department of Microsystems Engineering (IMTEK), Pennsylvania State University, Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506, USA, Massachusetts Institute of Technology, University of Minnesota, Pennsylvania State Univ, University of Maryland, Towson University, Department of Physics, Villanova University, University of Virginia, Boston University, Univ of Maryland-College Park, Harvard University, The Pennsylvania State Unversity, University of Wisconsin-Madison, McMaster University, California State University - Long Beach, National Chiao Tung University, National Chiao Tung University, Taiwan, Ohio University, University of Rennes, UMR CNRS 6251, Rennes, France, University of Bordeaux, UMR 5804, Floirac, France, University of Bordeaux, UMR 5255, Talence, France, Sandia National laboratories, Livermore, CA, Department of Chemistry, West Virginia University, Morgantwon, WV, The Pennsylvania State University, University of Toronto, Departamento de F\'isica, Facultad de Ciencias, Universidad de Chile, Casilla 653, Santiago, Chile, Cinvestav-Unidad Queretaro, Queretaro-76230, Mexico, Department of Physics and Astronomy, West Virginia University, Morgantown, WV-26505-6315, USA, The University of Arizona, TU Dortmund, Dortmund, Naval Air Warfare Center - Aircraft Division