Magnetic studies of S=1/2 kagom\'{e} lattice single crystals

ORAL

Abstract

The Zn-paratacamite mineral family, Zn$_{x}$Cu$_{4-x}$(OH)$_{6}$Cl$_{2}$, presents a promising system for studies of frustrated magnetism on a S=1/2 kagom\'{e} lattice. Here we report a new synthesis method, by which high quality single crystals of Zn-paratacamite can be produced. The x = 1 mineral herbertsmithite is a spin-liquid candidate. This compound displays a magnetic susceptibility that is anisotropic at high temperatures. A small anisotropy is observed in specific heat measurements with magnetic field applied in-plane and normal-to-plane. Inelastic neutron scattering has been performed and we will discuss the observed structure factor in the context of various theoretical expectations.

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Authors

  • Tianheng Han

    MIT

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University

  • Richard D. Averitt

    Trinity College, Department of Physics, Joint appointment in Teacher Education, Wright State University, Graduate School of Education, University of Massachusetts Lowell, Littleton High School, Department of Physics, Boston College, Department of Physics and Applied Physics, University of Massachusetts Lowell, North Carolina State University, University of Massachusetts at Lowell, University of Massachusetts Lowell, Harvard Medical School, Massachusetts General Hospital, Boston, MA, Harvard University, Department of Chemistry University of Massachusetts Amherst, Center for Advanced Materials and Department of Plastics Engineering University of Massachusetts Lowell, Center for Advanced Materials and Department of Physics and Applied Physics University of Massachusetts Lowell, RMD Inc., Watertown MA, UMass Lowell, Lowell MA, Radiation Monitoring Devices Inc., Watertown, MA, USA, University of Massachusetts, Lowell, MA, USA, Argonne National Laboratory, Argonne, IL, USA, ANL, IL, UMass Lowell, Brown University / Department of Chemistry, Sciprint.org, Physics Department, LESIMS Laboratory, Badji Mokhtar University, 23000 Annaba, Algeria, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Physics Department, Boston University