Mobility Enhancement and Highly Efficient Gating of Monolayer MoS$_{2}$ Transistors with Polymer Electrolyte

POSTER

Abstract

We report electrical characterization of monolayer molybdenum disulfide (MoS$_{2})$ devices using a thin layer of polymer electrolyte consisting of poly(ethylene oxide) (PEO) and lithium perchlorate (LiClO$_{4})$ as both a contact-barrier reducer and channel mobility booster. We find that bare MoS$_{2}$ devices (without polymer electrolyte) fabricated on Si/SiO$_{2}$ have low channel mobility and large contact resistance, both of which severely limit the field-effect mobility of the devices. A thin layer of PEO/ LiClO$_{4}$ deposited on top of the devices not only substantially reduces the contact resistance but also boost the channel mobility, leading to dramatically enhancement of the field-effect mobility of the device. When the polymer electrolyte is used as a gate medium, the MoS$_{2}$ field-effect transistors exhibit excellent device characteristics such as a near ideal subthreshold swing and an on/off ratio of 10$^{6}$ as a result of the strong gate-channel coupling.

Authors

  • Ming-Wei Lin

    Wayne State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University

  • Oleg Popov

    Miami University, Chemistry Department, Penn State Univ., University Park, PA 16802, unaffiliated, Department of Materials Science and Engineering, Ohio State University Columbus, OH 43210, Department of Physics, Ohio State University, Columbus, OH 43210, Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201, Korea Institute of Science and Technology, University of Cincinnati, Miami University of Ohio, University of Michigan, University of Notre Dame, University of Nebraska-Lincoln, Wayne State University, University of Tennessee, National Technical University of Athens, The University of Tennessee, Kettering Univeristy, University of Michigan-Dearborn, FNAL, Harvard University, California State University, Department of Physics, Kettering University, Flint, Michigan, Department of Natural Sciences, University of Michigan-Dearborn, Applied Sciences Inc., Cedarville, Ohio, Oakland University, University of Stockholm, Arizona State University