An unusual way to control the surface doping of cuprate superconductors in Angular Resolved Photoemission Spectroscopy (ARPES) experiments.

ORAL

Abstract

We study the variation of the electronic properties at the surface of a high temperature superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta}$ (Bi2212) as a function of vacuum conditions in angle resolved photoemission spectroscopy (ARPES) experiments. Normally, under less than ideal vacuum conditions the carrier concentration of (Bi2212) increases with time due to the absorption of oxygen from CO2 and CO molecules that are prime contaminants present in ultra high vacuum (UHV) systems. We find that in a high quality vacuum environment at low temperatures, the surface of Bi2212 is quite stable (the carrier concentration remains constant), however at elevated temperatures the carrier concentration decreases due to the loss of oxygen atoms from the Bi-O layer. These two effects can be used to control the carrier concentration in-situ. Allowing us to probe the doping phase diagram of cuprates on a single sample. Support: Department of Energy DE-AC02-07CH11358 \& DE-AC02-98CH10886 and National Science Foundation DMR-0537588

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Authors

  • Ari D. Palczewski

    Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA

  • Michael Turner

    Illinois Institute of Technology, Bettendorf High School, Bettendorf, IA, Mississippi Bend Area Education Agency, Bettendorf, IA, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA, Max-Planck-Institut fuer Mikrostrukturphysik, Halle, Germany, CNRS, Universite Lyon I, France, Freie Universitaet Berlin, Germany, University of Jyvaskila, Finaland, Iowa State University/Ames Laboratory, Materials Science Division, Argonne National Laboratory and Department of Chemistry, Northwestern University, Materials Science Division, Argonne National Laboratory, Advanced Photon Source, Argonne National Laboratory, Ames Laboratory and Iowa State University, Indiana University, Illinois State University, University of Iowa, Louisiana State University, University of Warwick, Rutherford Appleton Laboratory, Coe College, University of Northern Iowa, Iowa State University and Ames Laboratory, University of Illinois, Ames Laboratory, University of Florida, Tulane University, The Department of Physics and The James Franck Institute, The University of Chicago, J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, Department of Physics, Augustana College, Sioux Falls, SD 57197, Intense Laser Physics Theory Unit, Illinois State University, Argonne National Laboratory, Dr, Drake University, Physics Department, Ocean University of China, Qingdao, Physics Department, Southern Illinois University Carbondale, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA, Department of Physics, The University of Texas at Austin, Austin, Texas 78712, USA, NEST-CNR-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy, University of New Hampshire Department of Physics, University of Chicago

  • Michael Turner

    Illinois Institute of Technology, Bettendorf High School, Bettendorf, IA, Mississippi Bend Area Education Agency, Bettendorf, IA, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA, Max-Planck-Institut fuer Mikrostrukturphysik, Halle, Germany, CNRS, Universite Lyon I, France, Freie Universitaet Berlin, Germany, University of Jyvaskila, Finaland, Iowa State University/Ames Laboratory, Materials Science Division, Argonne National Laboratory and Department of Chemistry, Northwestern University, Materials Science Division, Argonne National Laboratory, Advanced Photon Source, Argonne National Laboratory, Ames Laboratory and Iowa State University, Indiana University, Illinois State University, University of Iowa, Louisiana State University, University of Warwick, Rutherford Appleton Laboratory, Coe College, University of Northern Iowa, Iowa State University and Ames Laboratory, University of Illinois, Ames Laboratory, University of Florida, Tulane University, The Department of Physics and The James Franck Institute, The University of Chicago, J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, Department of Physics, Augustana College, Sioux Falls, SD 57197, Intense Laser Physics Theory Unit, Illinois State University, Argonne National Laboratory, Dr, Drake University, Physics Department, Ocean University of China, Qingdao, Physics Department, Southern Illinois University Carbondale, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA, Department of Physics, The University of Texas at Austin, Austin, Texas 78712, USA, NEST-CNR-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy, University of New Hampshire Department of Physics, University of Chicago

  • Michael Turner

    Illinois Institute of Technology, Bettendorf High School, Bettendorf, IA, Mississippi Bend Area Education Agency, Bettendorf, IA, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA, Max-Planck-Institut fuer Mikrostrukturphysik, Halle, Germany, CNRS, Universite Lyon I, France, Freie Universitaet Berlin, Germany, University of Jyvaskila, Finaland, Iowa State University/Ames Laboratory, Materials Science Division, Argonne National Laboratory and Department of Chemistry, Northwestern University, Materials Science Division, Argonne National Laboratory, Advanced Photon Source, Argonne National Laboratory, Ames Laboratory and Iowa State University, Indiana University, Illinois State University, University of Iowa, Louisiana State University, University of Warwick, Rutherford Appleton Laboratory, Coe College, University of Northern Iowa, Iowa State University and Ames Laboratory, University of Illinois, Ames Laboratory, University of Florida, Tulane University, The Department of Physics and The James Franck Institute, The University of Chicago, J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, Department of Physics, Augustana College, Sioux Falls, SD 57197, Intense Laser Physics Theory Unit, Illinois State University, Argonne National Laboratory, Dr, Drake University, Physics Department, Ocean University of China, Qingdao, Physics Department, Southern Illinois University Carbondale, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA, Department of Physics, The University of Texas at Austin, Austin, Texas 78712, USA, NEST-CNR-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy, University of New Hampshire Department of Physics, University of Chicago

  • Michael Turner

    Illinois Institute of Technology, Bettendorf High School, Bettendorf, IA, Mississippi Bend Area Education Agency, Bettendorf, IA, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA, Max-Planck-Institut fuer Mikrostrukturphysik, Halle, Germany, CNRS, Universite Lyon I, France, Freie Universitaet Berlin, Germany, University of Jyvaskila, Finaland, Iowa State University/Ames Laboratory, Materials Science Division, Argonne National Laboratory and Department of Chemistry, Northwestern University, Materials Science Division, Argonne National Laboratory, Advanced Photon Source, Argonne National Laboratory, Ames Laboratory and Iowa State University, Indiana University, Illinois State University, University of Iowa, Louisiana State University, University of Warwick, Rutherford Appleton Laboratory, Coe College, University of Northern Iowa, Iowa State University and Ames Laboratory, University of Illinois, Ames Laboratory, University of Florida, Tulane University, The Department of Physics and The James Franck Institute, The University of Chicago, J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, Department of Physics, Augustana College, Sioux Falls, SD 57197, Intense Laser Physics Theory Unit, Illinois State University, Argonne National Laboratory, Dr, Drake University, Physics Department, Ocean University of China, Qingdao, Physics Department, Southern Illinois University Carbondale, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA, Department of Physics, The University of Texas at Austin, Austin, Texas 78712, USA, NEST-CNR-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy, University of New Hampshire Department of Physics, University of Chicago

  • Michael Turner

    Illinois Institute of Technology, Bettendorf High School, Bettendorf, IA, Mississippi Bend Area Education Agency, Bettendorf, IA, Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA, Max-Planck-Institut fuer Mikrostrukturphysik, Halle, Germany, CNRS, Universite Lyon I, France, Freie Universitaet Berlin, Germany, University of Jyvaskila, Finaland, Iowa State University/Ames Laboratory, Materials Science Division, Argonne National Laboratory and Department of Chemistry, Northwestern University, Materials Science Division, Argonne National Laboratory, Advanced Photon Source, Argonne National Laboratory, Ames Laboratory and Iowa State University, Indiana University, Illinois State University, University of Iowa, Louisiana State University, University of Warwick, Rutherford Appleton Laboratory, Coe College, University of Northern Iowa, Iowa State University and Ames Laboratory, University of Illinois, Ames Laboratory, University of Florida, Tulane University, The Department of Physics and The James Franck Institute, The University of Chicago, J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, KS 66506, Department of Physics, Augustana College, Sioux Falls, SD 57197, Intense Laser Physics Theory Unit, Illinois State University, Argonne National Laboratory, Dr, Drake University, Physics Department, Ocean University of China, Qingdao, Physics Department, Southern Illinois University Carbondale, Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011, Department of Physics and Astronomy, University of Missouri, Columbia, Missouri 65211, USA, Department of Physics, The University of Texas at Austin, Austin, Texas 78712, USA, NEST-CNR-INFM and Scuola Normale Superiore, I-56126 Pisa, Italy, University of New Hampshire Department of Physics, University of Chicago