X-ray diffraction experiments on the Materials in Extreme Conditions (MEC) LCLS x-ray FEL beamline

ORAL

Abstract

The experiments described here were conducted on the MEC beamline hutch at the SLAC Linac Coherent Light Source. A 10 ns 527 nm laser pulse was used to shock compress 60-100 $\mu$m thick NaCl and Graphite samples. LCLS x-rays (40 fs, 8 keV), scattered off the shocked sample, were recorded on several pixel array detectors positioned downstream. The diffracted x-ray pattern allows us to determine changes in crystal structure at Mbar pressures and over nanosecond timescales. In this talk we detail the experimental setup, the current capabilities of the MEC laser and the considerations for optimizing the target design. We will describe the wave interactions within the shock-compressed target and the use of a 1D hydrocode to describe the pressure, temperature and density conditions within the target assembly as a function of time and Lagrangian position. We present observations of the B1-B2 phase transition in NaCl and subsequent back transformation during release to ambient pressure, and compare these findings to gas gun and static data. We also present results from a preliminary study of the shock-induced graphite to diamond transformation.

Authors

  • Raymond Smith

    Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab

  • Dayne Fratanduono

    Lawrence Livermore National Laboratory

  • June Wicks

    Princeton University

  • Thomas Duffy

    Princeton University

  • Hae Ja Lee

    LCLS, SLAC, Stanford Linear Accelerator

  • Eduardo Granados

    SLAC National Laboratory, Stanford Linear Accelerator

  • Philip Heimann

    SLAC National Laboratory, Stanford Linear Accelerator

  • Arianna Gleason

    Los Alamos National Laboratory

  • Cindy Bolme

    Los Alamos National Laboratory, Los Alamos National Lab

  • Damian Swift

    Lawrence Livermore National Laboratory

  • Federica Coppari

    Lawrence Livermore National Laboratory, LLNL

  • Jon Eggert

    Lawrence Livermore Natl Lab, Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab

  • Gilbert Collins

    Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab