X-ray diffraction experiments on the Materials in Extreme Conditions (MEC) LCLS x-ray FEL beamline
ORAL
Abstract
The experiments described here were conducted on the MEC beamline hutch at the SLAC Linac Coherent Light Source. A 10 ns 527 nm laser pulse was used to shock compress 60-100 $\mu$m thick NaCl and Graphite samples. LCLS x-rays (40 fs, 8 keV), scattered off the shocked sample, were recorded on several pixel array detectors positioned downstream. The diffracted x-ray pattern allows us to determine changes in crystal structure at Mbar pressures and over nanosecond timescales. In this talk we detail the experimental setup, the current capabilities of the MEC laser and the considerations for optimizing the target design. We will describe the wave interactions within the shock-compressed target and the use of a 1D hydrocode to describe the pressure, temperature and density conditions within the target assembly as a function of time and Lagrangian position. We present observations of the B1-B2 phase transition in NaCl and subsequent back transformation during release to ambient pressure, and compare these findings to gas gun and static data. We also present results from a preliminary study of the shock-induced graphite to diamond transformation.
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Authors
Raymond Smith
Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab
Dayne Fratanduono
Lawrence Livermore National Laboratory
June Wicks
Princeton University
Thomas Duffy
Princeton University
Hae Ja Lee
LCLS, SLAC, Stanford Linear Accelerator
Eduardo Granados
SLAC National Laboratory, Stanford Linear Accelerator
Philip Heimann
SLAC National Laboratory, Stanford Linear Accelerator
Arianna Gleason
Los Alamos National Laboratory
Cindy Bolme
Los Alamos National Laboratory, Los Alamos National Lab
Damian Swift
Lawrence Livermore National Laboratory
Federica Coppari
Lawrence Livermore National Laboratory, LLNL
Jon Eggert
Lawrence Livermore Natl Lab, Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab
Gilbert Collins
Lawrence Livermore National Laboratory, LLNL, Lawrence Livermore National Lab