Stabilizing Room-Temperature Superconductivity in Hydrides by Nonequilibrium Driving

ORAL

Abstract

Metallic hydrogen and hydride materials are promising candidates to realize room-temperature superconductivity. Due to the high phonon frequency and intermediate coupling strength, the transition temperatures of various high-pressure hydrides have been predicted to be above 250 K, which experiments have further verified. To further increase the transition temperature above room temperature, we propose a dynamic approach, which can be realized by driving hydrides with mid-IR lasers. In the steady state driven by light, we simulate the increase of the density of states (DOS) via a combined Floquet and first-principles simulation. The increased DOS gives rise to the electron-phonon coupling constant λ for materials at all pressures, which increases the Tc based on the Migdal-Eliashberg and McMillan-Allen-Dynes theory. Using first-principles simulations and realistic pump conditions, we demonstrate that the transition temperature of LaH10 can be increased above the room temperature.

*This work is supported by the Air Force Office of Scientific Research Young Investigator Program under grant FA9550-23-1-0153. W.-C.C. and Y.W. also acknowledge support from the National Science Foundation (NSF) award DMR-2132338. A.D.S acknowledges support from the NSF awards No. OIA-2148653 and DMR-2142801. Simulation results were obtained using the Frontera computing system at the Texas Advanced Computing Center. Frontera is made possible by NSF Award No. OAC-1818253.

Presenters

  • Chendi Xie

    • Clemson University

Authors

  • Chendi Xie

    • Clemson University
  • Adam D. Smith

    • University of Alabama at Birmingham
  • Haoran Yan

    • Emory University
  • Wei-Chih Chen

    • Clemson University
  • Yao Wang

    • Clemson University
    • Emory University