Spin Excitation Continuum in the Exactly Solvable Triangular-Lattice Spin Liquid CeMgAl<sub>11</sub>O<sub>19</sub>

ORAL

Abstract

In magnetically ordered insulators, elementary quasiparticles manifest as spin waves - collective motions of localized magnetic moments propagating through the lattice - observed via inelastic neutron scattering. In effective spin-1/2 systems where geometric frustrations suppress static magnetic order, spin excitation continua can emerge, either from degenerate classical spin ground states or from entangled quantum spins characterized by emergent gauge fields and deconfined fractionalized excitations. Comparing the spin Hamiltonian with theoretical models can unveil the microscopic origins of these zero-field spin excitation continua. Here, we use neutron scattering to study spin excitations of the two-dimensional (2D) triangular-lattice effective spin-1/2 antiferromagnet CeMgAl11O19. Analyzing the spin waves in the field-polarized ferromagnetic state, we find that the spin Hamiltonian is close to an exactly solvable 2D triangular-lattice XXZ model, where degenerate 120 ordered ground states - umbrella states - develop in the zero temperature limit. We then find that the observed zero-field spin excitation continuum matches the calculated ensemble of spin waves from the umbrella state manifold, and thus conclude that CeMgAl11O19 is the first example of an exactly solvable spin liquid on a triangular lattice where the spin excitation continuum arises from the ground state degeneracy.

*US DOE BESRobert A. Welch FoundationQuantum Materials Synthesis (cQMS), funded by the Gordon and Betty Moore Foundation’s EPiQS initiativeSimons Collaboration on Ultra-Quantum MatterNational Natural Science Foundation of ChinaNational Research Foundation of Korea (NRF), Ministry of Science and ICTMLF of J-PARC proposal No.2022B0242SNS, a DOE Office of Science by ORNL

Publication: arXiv:2408.15957

Presenters

  • Bin Gao

    • Rice University

Authors

  • Bin Gao

    • Rice University
  • Tong Chen

    • Johns Hopkins University
  • Chunxiao Liu

    • University of California, Berkeley
  • Mason L Klemm

    • Rice University
  • Shu Zhang

    • Max Planck Institute for the Physics of Complex Systems
  • Zhen Ma

    • Hubei Normal University
  • Xianghan Xu

    • University of Minnesota, Twin Cities
    • Princeton University
  • Choongjae Won

    • Pohang Univ of Sci & Tech
  • Gregory T McCandless

    • Baylor University
  • Naoki Murai

    • Japan Atomic Energy Agency
  • Seiko Ohira-Kawamura

    • Japan Atomic Energy Agency
  • Stephen John Moxim

    • National Institute of Standards and Technology (NIST)
  • Jason Ryan

    • National Institute of Standards and Technology (NIST)
  • Xiaozhou Huang

    • Argonne National Laboratory
  • Xiaoping Wang

    • Oak Ridge National Laboratory
  • Julia Y Chan

    • Baylor Univeristy
    • Baylor University
    • Balor University
  • Sang-Wook Cheong

    • Rutgers University
  • Oleg V Tchernyshyov

    • Johns Hopkins University
  • Leon Balents

    • University of California, Santa Barbara
  • Pengcheng Dai

    • Rice University