Imaging stress and magnetsm at high pressures using quamtum sensors in a two-dimensional material

ORAL

Abstract

Pressure provides a powerful toolbox for altering material properties, leading to the discovery of novel phases and transitions. To investigate two-dimensional (2D) materials under hydrostatic pressure, local sensors near the target materials provide critical insights into their behavior. In this work, we demonstrate the capability to image mechanical stress and magnetism inside a diamond anvil cell, by directly transferring the hexagonal boron nitride flakes containing boron-vacancy (VB) centers. For stress, we find that the susceptibility of VB centers is over three times greater than that of their three-dimensional counterpart --- nitrogen-vacancy centers in diamond, allowing for precise stress measurement. For magnetism, we utilize VB centers to explore the pressure tuning of magnetism in the room temperature 2D magnet, chromium telluride. Our work opens new avenues for probing pressure-dependent phenomena in heterogeneous materials with embedded quantum sensors.

*Shixiong Zhang acknowledges support from NSF DMR-2327826James Edgar acknowledges support from the Office of Naval Research, Award N00014-22-1-2582. The neutron irradiation of hBN was supported by the U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-05ID14517 as part of Nuclear Science User Facilities award #23-4547

Presenters

  • Guanghui He

    • Washington University, St. Louis
    • Washington University in St. Louis

Authors

  • Guanghui He

    • Washington University, St. Louis
    • Washington University in St. Louis
  • Ruotian Gong

    • Washington University in St. Louis
  • Zhipan Wang

    • Harvard University
    • Harvard Univeristy
  • Zhongyuan Liu

    • Washington University in St. Louis
  • Ariana Lerena Riofrio

    • Santa Clara University
  • Yinyao Shi

    • Washington University, St. Louis
  • Changyu Yao

    • Washington University, St. Louis
  • Mingfeng Chen

    • Washington University in St. Louis
    • Washington University in St Louis
  • Zackary R Rehfuss

    • Washington University, St. Louis
  • Jeonghoon Hong

    • Indiana University Bloomington
  • Thomas Poirier

    • Kansas State University
  • Sheng Ran

    • Washington University, St. Louis
  • Xi Wang

    • WUSTL
    • Washington University in St Louis
    • Washington University
  • James Edgar

    • Kansas State University
  • Shixiong Zhang

    • Indiana University Bloomington
  • Norman Y Yao

    • Harvard University
  • Chong Zu

    • Washington University, St. Louis