Quantum Sensing of Spin Dynamics in 2D Antiferromagnets using Boron Vacancies in hBN

ORAL

Abstract

We report studies of widely dispersed boron vacancies (BV⁻) in thin hexagonal boron nitride (hBN) for enabling high sensitivity optical detection of antiferromagnetic resonance in van der Waals based antiferromagnets (AFMs). BV⁻ centers provide a promising platform for probing spin dynamics in low-dimensional magnetic systems given the ease with which hBN flakes are integrated with atomically thin layers of two-dimensional magnets. This detection mechanism relies on the enhancement of the color-center spin relaxation rate by the dipole field fluctuations arising from magnons generated by Néel vector dynamics in AFMs. Néel vector dynamics can be driven by resonant applied microwave fields or by magnetization switching, making this a potentially powerful platform for understanding dynamical phenomena in AFMs, which is important for spintronic applications requiring efficient Néel vector manipulation in emerging AFM systems.

*This research was primarily supported by the Center for Emergent Materials, an NSF MRSEC, under award number DMR-2011876. Partial funding by the NanoSystems Laboratory shared facility used in this research was provided by the Center for Emergent Materials, an NSF MRSEC under award number DMR-2011876

Publication: Das, Shekhar, Alex L. Melendez, I-Hsuan Kao, Janeth A. García-Monge, Daniel Russell, Jiahan Li, Kenji Watanabe et al. "Quantum Sensing of Spin Dynamics Using Boron-Vacancy Centers in Hexagonal Boron Nitride." Physical Review Letters 133, no. 16 (2024): 166704.

Presenters

  • Janeth A García-Monge

    • The Ohio State University

Authors

  • Janeth A García-Monge

    • The Ohio State University
  • Francisco Ayala Rodriguez

    • Ohio State University
  • I-Hsuan Kao

    • Carnegie Mellon University
  • Ravi Kumar Bandapelli

    • Carnegie Mellon University
  • Denis V Pelekhov

    • Ohio State University
  • Simranjeet Singh

    • Carnegie Mellon University
  • P Chris Hammel

    • Ohio State University