Quantum entanglement and quantum geometry measured with inelastic X-ray scattering

ORAL

Abstract

Using previously collected inelastic X-ray scattering (IXS) spectra, we investigated the quantum geometry and quantum information in the large-gap insulator, LiF. In this talk, I will describe how using sum rules for the density-density response function measured in IXS, we computed the quantum Fisher information of the equilibrium density matrix of LiF associated with density perturbations. Further, I will describe how, by exploiting universal relations between the quantum Fisher information, the optical conductivity, and the quantum metric tensor, we extrapolated the diagonal (h,k,l) = (1,0,0) component of the quantum metric of LiF, known as the quantum weight. I will show a comparison between results and recently proposed bounds on the quantum weight, which shows that LiF resides near the lower bound, supporting the general understanding of this material as a highly localized, ionic insulator. Our work serves as a proof-of-principle that IXS techniques can be used to quantify state-of-the-art quantum geometric quantities of materials.

*This work was primarily supported by the Center for Quantum Sensing and Quantum Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under award DE-SC0021238. P.A. gratefully acknowledges additional support from the EPiQS program of the Gordon and Betty Moore Foundation, grant GBMF9452. The theoretical work of B.B. on wavefunction geometry was additionally supported by the Alfred P. Sloan foundation, and the National Science Foundation under grant DMR-1945058. IXS measurements at the Advanced Photon Source were supported by DOE grant DE-AC02-06CH11357. D.B. was supported in part by the A.C. Anderson Undergraduate Research Scholar Award, Department of Physics, University of Illinois Urbana-Champaign.

Publication: arXiv:2409.15583

Presenters

  • David Balut

    • University of Illinois at Urbana-Champaign
    • University of Illinois at Urbana Champaign

Authors

  • David Balut

    • University of Illinois at Urbana-Champaign
    • University of Illinois at Urbana Champaign
  • Peter Abbamonte

    • University of Illinois at Urbana-Champaign
  • Barry Bradlyn

    • University of Illinois at Urbana-Champaign
    • University of Illinois Urbana-Champaign