Local imaging of ferromagnetism and topology in twisted bilayer MoTe2

ORAL

Abstract

Bilayer MoTe2 has been recently shown to host Fractional Chern Insulators at zero magnetic field. Here, we use a nanoscale superconducting sensor to map the magnetic fringe fields in twisted bilayers of MoTe2. In the twist angle range from 3.5 to 3.9 degrees, we observe oscillations in the local magnetic field associated with fillings ν=−1,−2/3,−3/5,−4/7 and −5/9 of the first moiré hole band, consistent with the formation of FCIs at these fillings. By quantitatively reconstructing the magnetization, we determine the local thermodynamic gaps of the most robust FCI state at ν=−2/3 to be as large as 7 meV. Spatial mapping of the charge density- and displacement field-tuned magnetic phase diagram further allows us to characterize sample disorder, which we find to be dominated by both inhomogeneity in the effective unit cell area as well as inhomogeneity in the band edge offset and bound electric dipole moment.

For smaller twist angles ranging from 2.1 to 2.7 degrees, we observe FCIs in a similar sequence, albeit with reduced gap size. We also observe a ferromagnetic signal associated with a state at v=-3. We discuss these results in the context of recent theoretical and experimental literature concerning the nature of correlated and topological phases in this system.

*Work at UCSB was primarily supported by the Army Research Office under award W911NF-20-2-0166. E.R. and O.S. acknowledge support by the National Science Foundation through Enabling Quantum Leap: Convergent Accelerated Discovery Foundries for Quantum Materials Science, Engineering and Information (Q-AMASE-i) award number DMR-1906325. A.F.Y. acknowledges additional support by the Gordon and Betty Moore Foundation EPIQS program under award GBMF9471. A.F.Y. also acknowledges the support of the W. M. Keck Foundation under award SB190132 for the development of SQUID microscopy techniques.

Publication: Redekop E. et al "Direct magnetic imaging of fractional Chern insulators in twisted MoTe2 with a superconducting sensor", Nature, 2024

Presenters

  • Evgeny Redekop

    • University of California, Santa Barbara

Authors

  • Evgeny Redekop

    • University of California, Santa Barbara
  • Canxun Zhang

    • University of California, Santa Barbara
  • Heonjoon Park

    • University of Washington
  • Jiaqi Cai

    • University of Washington
  • Eric Anderson

    • University of Washington
  • Owen I Sheekey

    • University of California, Santa Barbara
  • Trevor B Arp

    • University of California, Santa Barbara
  • Grigory Babikyan

    • University of California, Santa Barbara
  • Samuel Salters

    • University of California, Santa Barbara
  • Kenji Watanabe

    • National Institute for Materials Science
    • NIMS
    • Research Center for Functional Materials, National Institute for Materials Science
    • Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Material Science, Tsukuba, Japan
    • National Institute of Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Takashi Taniguchi

    • National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute of Material Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Martin E Huber

    • University of Colorado, Denver
  • Xiaodong Xu

    • University of Washington
  • Andrea F Young

    • University of California, Santa Barbara
    • University of California Santa Barbara
    • University of California at Santa Barbara