Orbital-to-Spin Ratio of Dynamic Magnetization in Co/Pt

ORAL

Abstract

Recent theoretical work suggests that ferromagnets can generate orbital angular momentum through resonant magnetization dynamics involving both spin and orbital components [1,2]. X-ray magnetic circular dichroism measure the ratio of orbital-to-spin moment (μLS) in the dynamic magnetization of Co/Pt, a material combination known for strong spin-orbit coupling. We aim to explore whether orbital and spin magnetization dynamics can be distinct.

The dynamic X-ray transmission response of the FMR-driven Co magnetization precession at various photon energies was recorded, yielding the dynamic XMCD at Co L3,2 edges. By applying the XMCD sum rule analysis, we find (μLS)dynamic = 0.107 ± 0.002. This is about 5% more than (μLS)static = 0.102 ± 0.002 obtained from the static XMCD. The error bars for (μLS)dynamic and (μLS)static account for uncertainty due to background signal processing. The smaller (μLS)static compared to (μLS)dynamic could imply faster spin dissipation than orbital dissipation in Co interfaced with Pt. Our research contributes to understanding non-equilibrium orbital and spin angular moment, crucial for advanced "spin-orbitronic" devices.

[1] D. Go et al., arXiv:2309.14817 (2023).

[2] H. Hayashi et al., Nature Electronics, 1-7 (2024).

*We acknowledge the following funding bodies for their support:NSF Grant No. ECCS-2144333; AFOSR Grant No. FA9550-21-1-0365; NSF Grant No. ECCS-2236160; DoE BES Contract No. DE-AC02-05-CH11231.

Presenters

  • Omolara A Bakare

    • Virginia Tech

Authors

  • Omolara A Bakare

    • Virginia Tech
  • Galen T Street

    • Virginia Polytechnic Institute
    • Virginia Tech
  • Rachel E Maizel

    • Virginia Tech
  • Christoph Klewe

    • Lawrence Berkeley National Laboratory
  • Satoru Emori

    • Virginia Tech