The real-time Dyson expansion: many-body physics with mean-field cost

ORAL

Abstract

Time-resolved photoemission spectroscopy is the key technique to probe the real-time non-equilibrium dynamics of electronic states. However its theoretical prediction remains a challenge. Typically including many-body correlations (crucial for accurate predictions of non-equilibrium phenomena), requires solving the Kadanoff-Baym equations, which scale cubically in the number of time-steps. This poor scaling makes them prohibitively expensive in many practical situations. In a recent paper we have introduced a new method, called the RT-DE, that allows for the inclusion of dynamical correlations in the spectral function while maintaining the same scaling in the number of time steps as for mean-field approaches (effectively linear). In this talk we will introduce the RT-DE methodology and then discuss an application studying the effect of dynamical correlations on band-gap renormalization in photo-excited semiconductors.

*This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research and Office of Basic Energy Sciences, Scientific Discovery through Advanced Computing (SciDAC) program under Award Number DE-SC0022198. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 using NERSC award BES-ERCAP0029462

Publication: Cian Reeves and Vojtech Vlcek, A Real-time Dyson Expansion Scheme: Efficient Inclusion of Dynamical Correlations in Non-equilibrium Spectral Properties

Presenters

  • Cian Charles Reeves

    • University of California, Santa Barbara

Authors

  • Cian Charles Reeves

    • University of California, Santa Barbara
  • Vojtech Vlcek

    • University of California, Santa Barbara