Nernst effect induced by a Fermi surface nesting instability in a magnetic Weyl semimetal NdAlSi

ORAL

Abstract

The thermoelectric Nernst effects are sensitive to details of the electronic structure around the Fermi energy, including the quantum-mechanical Berry phase of the conduction electrons. Here, we quantitatively demonstrate that Nernst effects are significantly enhanced when the Fermi surface has 'hot spots' of scattering time, using a correlated topological semimetal with high carrier mobility in presence of magnetic fluctuations [R. Yamada, Phys. Rev. X (2024)]. Supported by detailed ab-initio calculations and clear quantum oscillations, our thermoelectric measurements on a single crystalline sample of a magnetic Weyl semimetal NdAlSi reveal a drastic enhancement of the Nernst effect in vicinity of a magnetic ordering instability. This work paves the way in the research field of thermoelectric for correlation-driven thermoelectric response independent of a material's carrier density, i.e. in metals, semimetals, and semiconductors with large mobility.

*This work was supported by JSPS KAKENHI Grants No. JP21K13877, No. JP22H04463, No. JP22K20348, No. JP23H05431, and No. JP23K13057, JST CREST Grants No. JPMJCR1874, JPMJCR20T1 (Japan), JST FOREST Grant No. JPMJFR2238 (Japan), the Fujimori Science and Technology Foundation, the New Materials and Information Foundation, the Murata Science Foundation, the Mizuho Foundation for the Promotion of Sciences, the Yamada Science Foundation, the Hattori Hokokai Foundation, the Iketani Science and Technology Foundation, the Mazda Foundation, the Casio Science Promotion Foundation, the Takayanagi Foundation, the Foundation for Promotion of Material Science Technology of Japan (MST Foundation), and the Yashima Environment Technology Foundation.

Publication: R. Yamda et al., Physical Review X 14, 021012 (2024)

Presenters

  • Rinsuke Yamada

    • The Univesity of Tokyo
    • Univ of Tokyo

Authors

  • Rinsuke Yamada

    • The Univesity of Tokyo
    • Univ of Tokyo
  • Takuya Nomoto

    • Univ of Tokyo
    • Tokyo Metropolitan University
    • Tokyo Metropolitan Univ.
  • Atsushi Miyake

    • Tohoku University
  • Toshihiro Terakawa

    • Univ of Tokyo
  • Akiko Kikkawa

    • RIKEN CEMS
    • RIKEN
  • Ryotaro Arita

    • Univ of Tokyo
    • Univ. of Tokyo, RIKEN CEMS
  • Masashi Tokunaga

    • ISSP, University of Tokyo
    • Univ of Tokyo
  • Yasujiro Taguchi

    • RIKEN
    • RIKEN CEMS
    • RIKEN Center for Emergent Matter Science (CEMS)
  • Yoshinori Tokura

    • RIKEN Center for Emergent Matter Science (CEMS), Department of Applied Physics and Quantum-Phase Electronics Center (QPEC), The University of Tokyo
    • Univ of Tokyo
    • The University of Tokyo, RIKEN Center for Emergent Matter Science (CEMS), Tokyo college, The University of Tokyo
    • RIKEN Center for Emergent Matter Science (CEMS); Department of Applied Physics and Quantum-Phase Electronics Center (QPEC), Univ. of Tokyo; Tokyo College, Univ. of Tokyo
    • RIKEN Center for Emergent Matter Science (CEMS), Department of Applied Physics, Quantum-Phase Electronics Center (QPEC) and Tokyo College, University of Tokyo
  • Max Hirschberger

    • Univ of Tokyo
    • University of Tokyo