Direct Visualization of a Disorder Driven Smectic Electronic Phase in Dirac Nodal Line Semimetal GdSbTe

ORAL

Abstract

Electronic liquid crystal (ELC) phases are spontaneous symmetry breaking states believed to arise from strong electron correlation in quantum materials such as cuprates and iron pnictides. Here, we report a direct observation of an ELC phase in a weakly correlated Dirac nodal line (DNL) semimetal GdSbxTe2-x. Electronic nanostructures consisting of incommensurate smectic charge modulation and intense local unidirectional nanostructure are visualized by using spectroscopic imaging - scanning tunneling microscopy. As topological materials with symmetry protected Dirac or Weyl fermions are mostly weakly correlated, the discovery of such an ELC phase are anomalous and raise questions on the origin of their emergence. Specifically, we demonstrate how chemical substitution generates these symmetry breaking phases before the system undergoes a charge density wave - orthorhombic structural transition. Our results highlight the importance of impurities in realizing ELC phases and present a new material platform for exploring the interplay among quenched disorder, topology and electron correlation.

*This work is supported by National Science and Technology Council (NSTC) in Taiwan, by Academia Sinica (AS-iMATE-113-12, AS-iMATE-113-15) and by National Taiwan University under Grant No. NTU-CC-113L891601 (Y.J.K.). T.-R.C. was supported by the 2030 Cross-Generation Young Scholars Program from NSTC, National Cheng Kung University (NCKU), Taiwan, and National Center for Theoretical Sciences, Taiwan. This research was supported, in part by Higher Education Sprout Project, Ministry of Education to the Headquarters of University Advancement at NCKU. A.D. acknowledges partial support by the National Science Foundation Materials Research Science and Engineering Center program through the UT Knoxville Center for Advanced Materials and Manufacturing (DMR-2309083). T.M.C. is grateful for the support of Golden-Jade Fellowship from Kenda Foundation.

Publication: https://arxiv.org/abs/2402.18893

Presenters

  • Tien-Ming Chuang

    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
    • Academia Sinica

Authors

  • Tien-Ming Chuang

    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
    • Academia Sinica
  • Balaji Venkatesan

    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
  • Syu-You Guan

    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
    • Academia Sinica
  • Jen-Te Chang

    • California Institute of Technology
    • Caltech
  • Shiang-Bin Chiu

    • Department of Physics, University of Washington
  • Po-Yuan Yang

    • Department of Physics, National Cheng-Kung University, Tainan 701, Taiwan
  • Chih-Chuan Su

    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
  • Tay-Rong Chang

    • National Cheng Kung University
    • National Cheng Kung University, R.O.C.
  • Kalaivanan Raju

    • Academia Sinica
    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
  • Raman Sankar

    • Academia Sinica
    • Institute of Physics, Academia Sinica, Taipei 11529, Taiwan
  • Somboon Fongchaiya

    • Center for Condensed Matter Sciences, National Taiwan University, Taipei 10617, Taiwan
  • Ming-Wen Chu

    • Center for Condensed Matter Sciences, National Taiwan University, Taipei 10617, Taiwan
  • Chia-Seng Chang

    • Inst of Physics Academia Sinica
  • Guoqing Chang

    • Nanyang Technological University
  • Hsin Lin

    • Academia Sinica
  • Adrian Del Maestro

    • University of Tennessee
    • University of Tennessee-Knoxville
  • Ying-Jer Kao

    • National Taiwan University