Spin polarization detection via chirality-induced tunneling currents in layered semiconductors

ORAL

Abstract

Two-dimensional flat-band systems offer a platform for exploring emergent phenomena and correlated electronic states. In this talk, we investigate few-layer indium selenide (InSe), a material known for its remarkable optical, electrical, and thermoelectric properties, which hosts a van Hove singularity at the valence band edge without requiring twist angle manipulation. We demonstrate how tunneling photocurrents in gated semiconductors serve as an effective probe for the flat-band energy position, supported by ambipolar transport and photoluminescence measurements. A distinct change in tunneling mechanisms emerges near the van Hove singularity, allowing for its detection up to room temperature. Moreover, we study the interaction between light chirality and electron spins in InSe under a magnetic field, revealing an asymmetric tunneling response under circularly polarized light. This enables the electrical detection of light's chirality and confirms the theoretical prediction of spin-polarized hole accumulation at the flat valence band with increasing laser power. These findings provide new insights into flat-band physics and the interplay of chirality and spin, with potential applications in future technologies.

*We acknowledge the support of the Swiss National Science Foundation (grant nos 164015, 175822, 177007, P500PT_222337), the European Union's Horizon 2020 (8816030 (Graphene Flagship Core 3), the Deutsche Forschungsge-meinschaft SFB 1277 (Project-ID 314695032, projects B07 and B11) and SPP 2244 (Project No. 443416183).

Publication: [1] Pasquale, G., Lopriore, E., Sun, Z., Cernevics, K., Tagarelli, F., Yazyev, O., Kis, A. Electrical detection of the flat band dispersion in van der Waals field-effect structures, Nature Nanotechnology, 18, 1416–1422 (2023).
[2] Pasquale, G., Sun, Z., Migliato Marega, G., Watanabe, K., Taniguchi, T., Kis, A., Electrically tunable giant Nernst effect in two-dimensional van der Waals heterostructures, Nature Nanotechnology 19, 941–947 (2024).
[3] Pasquale, G., Faria Junior, P., Collette, E., Watanabe, K., Taniguchi, T., Fabian, J., Kis, A., Spin polarization detection via chirality-induced tunneling currents in indium selenide. (accepted).

Presenters

  • Gabriele Pasquale

    • Harvard University

Authors

  • Gabriele Pasquale

    • Harvard University
  • Paulo E. Faria Junior

    • University of Regensburg
  • Shun Feng

    • Heriot-Watt University
  • Kenji Watanabe

    • National Institute for Materials Science
    • NIMS
    • Research Center for Functional Materials, National Institute for Materials Science
    • Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Material Science, Tsukuba, Japan
    • National Institute of Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Takashi Taniguchi

    • National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute of Material Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Jaroslav Fabian

    • University of Regensburg
  • Andras Kis

    • Ecole Polytechnique Federale de Lausanne
    • École Polytechnique Fédérale de Lausanne