Spin polarization detection via chirality-induced tunneling currents in layered semiconductors
ORAL
Abstract
Two-dimensional flat-band systems offer a platform for exploring emergent phenomena and correlated electronic states. In this talk, we investigate few-layer indium selenide (InSe), a material known for its remarkable optical, electrical, and thermoelectric properties, which hosts a van Hove singularity at the valence band edge without requiring twist angle manipulation. We demonstrate how tunneling photocurrents in gated semiconductors serve as an effective probe for the flat-band energy position, supported by ambipolar transport and photoluminescence measurements. A distinct change in tunneling mechanisms emerges near the van Hove singularity, allowing for its detection up to room temperature. Moreover, we study the interaction between light chirality and electron spins in InSe under a magnetic field, revealing an asymmetric tunneling response under circularly polarized light. This enables the electrical detection of light's chirality and confirms the theoretical prediction of spin-polarized hole accumulation at the flat valence band with increasing laser power. These findings provide new insights into flat-band physics and the interplay of chirality and spin, with potential applications in future technologies.
*We acknowledge the support of the Swiss National Science Foundation (grant nos 164015, 175822, 177007, P500PT_222337), the European Union's Horizon 2020 (8816030 (Graphene Flagship Core 3), the Deutsche Forschungsge-meinschaft SFB 1277 (Project-ID 314695032, projects B07 and B11) and SPP 2244 (Project No. 443416183).
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Publication:[1] Pasquale, G., Lopriore, E., Sun, Z., Cernevics, K., Tagarelli, F., Yazyev, O., Kis, A. Electrical detection of the flat band dispersion in van der Waals field-effect structures, Nature Nanotechnology, 18, 1416–1422 (2023). [2] Pasquale, G., Sun, Z., Migliato Marega, G., Watanabe, K., Taniguchi, T., Kis, A., Electrically tunable giant Nernst effect in two-dimensional van der Waals heterostructures, Nature Nanotechnology 19, 941–947 (2024). [3] Pasquale, G., Faria Junior, P., Collette, E., Watanabe, K., Taniguchi, T., Fabian, J., Kis, A., Spin polarization detection via chirality-induced tunneling currents in indium selenide. (accepted).
Presenters
Gabriele Pasquale
Harvard University
Authors
Gabriele Pasquale
Harvard University
Paulo E. Faria Junior
University of Regensburg
Shun Feng
Heriot-Watt University
Kenji Watanabe
National Institute for Materials Science
NIMS
Research Center for Functional Materials, National Institute for Materials Science
Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
Research Center for Functional Materials, National Institute of Material Science, Tsukuba, Japan
National Institute of Materials Science
Advanced Materials Laboratory, National Institute for Materials Science
Takashi Taniguchi
National Institute for Materials Science
International Center for Materials Nanoarchitectonics, National Institute for Materials Science
Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
International Center for Materials Nanoarchitectonics, National Institute of Material Science, Tsukuba, Japan
Advanced Materials Laboratory, National Institute for Materials Science