Nano-imaging of Plasmon polaritons of graphene on SrTiO<sub>3</sub> using terahertz scanning near-field optical microscope

ORAL

Abstract

The electrical and optoelectronic properties of graphene are significantly influenced by the underlying substrate. Replacing the conventional SiO₂/Si substrate with a high-dielectric, atomically smooth ferroelectric substrate such as SrTiO₃ dramatically changes the carrier densities dynamics in graphene. To explore the unique properties of surface plasmon polaritons (SPPs) in graphene on a dielectric substrate, we experimentally apply two advanced imaging techniques: nano-photocurrent mapping in magneto-scanning near-field optical microscopy (m-SNOM) and terahertz time-domain scanning near-field optical microscopy (THz-SNOM) with spacetime metrology. Utilizing THz-SNOM with fine spatial and temporal resolution, we investigate the charge density inhomogeneities and group velocities of SPPs, revealing key insights into the plasmonic behavior of 2D plasmons with a SrTiO₃ substrate.

*M.K.Liu acknowledges Gordon and Betty Moore Foundation DOI: 10.37807/gbmf12258 for supporting the development of polaritonic materials. Research on m-SNOM development is supported as part of Programmable Quantum Materials (Pro-QM), an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under award DE-SC0019443. M.K.L. also acknowledges support from the NSF Faculty Early Career Development Program under Grant No. DMR - 2045425.

Presenters

  • Zhenbing Dai

    • Stony Brook University (SUNY)

Authors

  • Zhenbing Dai

    • Stony Brook University (SUNY)
  • JiHoon Park

    • Stony Brook University (SUNY)
  • Shoujing Chen

    • Stony Brook University (SUNY)
  • Ran Jing

    • Brookhaven National Laboratory
    • Columbia University
  • Boyi Zhou

    • Columbia University
  • Lukas Wehmeier

    • Brookhaven National Laboratory (BNL)
  • Wenjun Zheng

    • Stony Brook University (SUNY)
  • Zijian Zhou

    • Stony Brook University (SUNY)
  • Suheng Xu

    • Columbia University
  • Yinan Dong

    • Columbia University
  • Ian wang

    • Stony Brook University(SUNY)
  • Tom Liu

    • Stony Brook University(SUNY)
  • Xu Du

    • Stony Brook University (SUNY)
  • Dmitri N Basov

    • Columbia University
  • Mengkun Liu

    • Stony Brook University (SUNY)