Discerning short- and long-range charge orders in YBa<sub>2</sub>Cu<sub>3</sub>O<sub>6+x</sub> using ultrafast resonant soft X-ray scattering

ORAL

Abstract

Time-resolved resonant soft X-ray scattering is emerging as a key technique for studying the interplay between order parameters in complex materials. Recent studies have shown a strong dynamical interaction between superconductivity and charge density waves (CDW) in cuprates. However, the photo-induced CDW dynamics in the non-superconducting state remain poorly understood. Here we present an ultrafast soft x-ray scattering study of the CDW dynamics in YBa2Cu3O6+x. The fluence-dependent response of the CDW peak shows clear saturation above a critical fluence ΦC, indicating complete quenching of the long-range order. Surprisingly, momentum scans reveal a persistent broad residual peak above ΦC. We compare this residual peak to the CDW signature well above the transition temperature and analyze the temporal evolution of the CDW momentum profile to understand the nature of these short-range correlations.

*The use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) under Contract No. DE-AC02-76SF00515. This work is supported in part by the Department of Energy, Laboratory Directed Research and Development funding, under contract DE-AC02-76SF00515.

Presenters

  • Choongwon Seo

    • SLAC National Accelerator Laboratory

Authors

  • Choongwon Seo

    • SLAC National Accelerator Laboratory
  • Fabio Boschini

    • INRS - Energie et Materiaux
  • Lingjia Shen

    • SLAC National Accelerator Laboratory
  • Alexander Nicolas Dominik Petsch

    • SLAC National Accelerator Laboratory
  • Vincent Esposito

    • SLAC national Accelerator Laboratory
  • Jake D Koralek

    • SLAC National Accelerator Laboratory
  • Georgi Dakovski

    • SLAC National Accelerator Laboratory
  • Andrea Damascelli

    • University of British Columbia
  • Eduardo H Da Silva Neto

    • Yale University
  • Joshua J Turner

    • SLAC National Accelerator Laboratory
  • Giacomo Coslovich

    • SLAC National Accelerator Laboratory