Metal capping for quality improvement of resonator – the art of choosing the right metal

ORAL

Abstract

Aluminum (Al) thin films have been widely used in superconducting circuits and for forming Josephson junctions due to their low kinetic inductance, stable oxide formation, and metal softness. However, they are prone to pinholes, allowing oxygen penetration through grain boundaries and impacting the metal-substrate interface. Increasing film thickness reduces oxidation by promoting larger grains.[1–3] Various pre-processing methods have been utilized to improve the interface characteristics, as the metal-substrate interface plays a critical role in the quality and performance of superconducting quantum devices. [4] To address these issues, we investigated a self-limiting oxidation metal as a capping layer to reduce oxidation at the aluminum-substrate interface. Capped aluminum films showed a crystal orientation shift from [111] to [002], indicating that the capping layer affects nucleation and growth, promoting a different orientation. We are examining how capping layer thickness impacts transition temperature and resonator quality factors and its role as an adhesive layer in altering aluminum's crystal orientation. We will present detailed interface characterizations and the performance of the resonator quality factor at the meeting. Detailed interface characterizations and resonator performance data will be presented.

*The National Research Foundation, Singapore, and A*STAR supported this research under its Quantum Engineering Programme (NRF2021-QEP2-02-P10 and NRF2021QEP2-03-P07).

Publication: [1] J. Biznárová et al., Mitigation of interfacial dielectric loss in aluminum-on-silicon superconducting qubits, Npj Quantum Inf. 10, 78 (2024).
[2] H. Takatsuji and T. Arai, Pinholes in Al thin films: their effects on TFT characteristics and a taguchi method analysis of their origins, Vacuum 59, 606 (2000).
[3] K. M. Law, S. Budhathoki, S. Ranjit, F. Martin, A. S. Thind, R. Mishra, and A. J. Hauser, Demonstration of nearly pinhole-free epitaxial aluminum thin films by sputter beam epitaxy, Sci. Rep. 10, 18357 (2020).
[4] D. S. Wisbey, J. Gao, M. R. Vissers, F. C. S. Da Silva, J. S. Kline, L. Vale, and D. P. Pappas, Effect of metal/substrate interfaces on radio-frequency loss in superconducting coplanar waveguides, J. Appl. Phys. 108, (2010).

Presenters

  • senthil kumar Karuppannan

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • NQFF, Institute of Materials Research and Engineering (IMRE), A*STAR
    • Institute of Materials Research and Engineering (IMRE)

Authors

  • senthil kumar Karuppannan

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • NQFF, Institute of Materials Research and Engineering (IMRE), A*STAR
    • Institute of Materials Research and Engineering (IMRE)
  • Rangga P Budoyo

    • Centre for Quantum Technologies, National University Singapore, Singapore, 117543, Republic of Singapore.
  • Nguyen H Long

    • Centre for Quantum Technologies, National University Singapore, Singapore, 117543, Republic of Singapore.
  • Naga Manikanta Kommanaboina

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • NQFF, Institute of Materials Research and Engineering (IMRE), A*STAR
    • Institute of Materials Research and Engineering, Technology and Research (A*STAR)
  • Guangxu Yan

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • Institute of Materials Research and Engineering (IMRE)
  • Rasanayagam S Kajen

    • Centre for Quantum Technologies, National University Singapore, Singapore, 117543, Republic of Singapore.
  • Nelson Lim C Beng

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • Institute of Materials Research and Engineering, Technology and Research (A*STAR)
  • Yap Lee K Sherry

    • NQFF, Institute of Materials Research and Engineering (IMRE)
    • Institute of Materials Research and Engineering, Technology and Research (A*STAR)
  • Rainer H Dumke

    • Centre for Quantum Technologies, National University Singapore, Singapore, 117543, Republic of Singapore.