Spontaneous Magnetic field and chiral superconductivity in BaPtAs<sub>1-x</sub>Sb<sub>x</sub> with honeycomb network

ORAL

Abstract

In recent years, a time-reversal symmetry-breaking superconducting (SC) state in which spontaneous magnetic field appears has attracted much attention. In materials with a so-called honeycomb network, the possibility of chiral d-wave superconductivity has been discussed [1]. Muon spin relaxation (μSR) is one of powerful tools for detecting spontaneous magnetic field.

In the layered pnictide BaPtAs1-xSbx with a honeycomb network, superconductivity appears over the entire range of x = 0 – 1.0 [2]. However, it has been unknown whether chiral d-wave superconductivity appears in this compound. Therefore, we performed μSR measurements on BaPtAs1-xSbx changing x widely [3].

It was found that the relaxation rate of muon spins increased below Tc = 1.7 K at x = 1.0, suggesting that spontaneous magnetic field is generated and time-reversal symmetry is broken. Moreover, the spontaneous magnetic field almost disappeared at x = 0.9, where a small amount of As was substituted for Sb, indicating that this superconductivity was weak to disorder. These suggest that the time-reversal symmetry-breaking SC state at x = 1.0 may have nodes on the SC gap. In the talk, I will compare these results with the band structure and Fermi surfaces obtained from the first-principles calculation and discuss the possibility of chiral d-wave superconductivity.

[1] P. K. Biswas et al. Phys. Rev. B 87, 180503(R) (2013).

[2] T. Ogawa et al., J. Phys. Soc. Jpn. 91, 123702 (2022).

[3] T. Adachi et al., submitted.

*This work was partly supported by JSPS KAKENHI Grant Number JP19H05823, JP20K03826, JP22H01182 and by JST SPRING, Grant Number JPMJSP2152.

Publication: "Spontaneous magnetic field and disorder effects in BaPtAs1−xSbx with honeycomb network", T. Adachi, T. Ogawa, Y. Komiyama, T. Sumura, Y. Saito-Tsuboi, T. Takeuchi, K. Mano, K. Manabe, K. Kawabata, T. Imazu, A. Koda, W. Higemoto, H. Okabe, J. G. Nakamura, T. U. Ito, R. Kadono, C. Baines, I. Watanabe, Y. Imai, J. Goryo, M. Nohara, and K. Kudo, submitted to Phys. Rev. B.

Presenters

  • Tadashi Adachi

    • Sophia University

Authors

  • Tadashi Adachi

    • Sophia University
  • Taiki Ogawa

    • Osaka University, Okayama University
  • Yota Komiyama

    • Sophia University
  • Takuya Sumura

    • Sophia University
  • Yuki Saito

    • Okayama University
  • Takaaki Takeuchi

    • Okayama University
  • Kohei Mano

    • Okayama University
  • Kaoru Manabe

    • Osaka University
  • Koki Kawabata

    • Sophia University
  • Tsuyoshi Imazu

    • Hirosaki University
  • Akihiro Koda

    • KEK
  • Wataru Higemoto

    • JAEA
  • Hirotaka Okabe

    • Tohoku University
  • Jumpei G Nakamura

    • KEK
  • Takashi U Ito

    • JAEA
  • Ryosuke Kadono

    • KEK, High Energy Accelerator Research Organization
    • KEK
  • Christopher Baines

    • Paul Scherrer Institute
    • PSI
  • Isao Watanabe

    • RIKEN
  • Yoshiki Imai

    • Okayama University of Science
  • Jun Goryo

    • Hirosaki University
  • Minoru Nohara

    • Hiroshima University
  • Kazutaka Kudo

    • Osaka University