Title: Correlated electronic states in MoSe<sub>2</sub> enabled by a periodic nanopatterned gate

ORAL

Abstract



Physical realizations of correlated electronic states have proven to be powerful tools in simulating quantum many-body interactions, altering electronic phase diagrams, and electronic band-engineering. Many of these systems have been enabled in recent years by transition metal dichalcogenides (TMDs), due in part to their enhanced Coulomb interactions and low-defect densities. Systems hosting correlated charge states are often realized by periodic moiré potentials that confine carriers to a superlattice. While these systems have proved fruitful, imprecise stacking techniques can lead to inconsistent moiré periodicities, and the states are geometrically constrained by the lattice structure of the moiré. I will present an alternative approach that enables customizable lattices to be engineered into monolayer MoSe2. Using nano-scale gate patterning, we defined a 40 nm periodic, 2D triangular lattice of etched holes into a graphene gate that was integrated into an MoSe2 heterostructure. Using gate-dependent, helicity-resolved differential reflectivity, we observe evidence of integer and fractional correlated states with enhanced magnetic interactions. We observed up to = 4 electron filling of the patterned lattice and enhanced Zeeman splitting that resulted in a maximum exciton g-factor of 20.

*Funding Acknowledgement: We acknowledge support from NSF Grant Nos. ECCS-2054572, ECCS-2428575, and AFOSR Grant Nos. FA9550-22-1-0312, FA9550-22-1-0113.

Presenters

  • Trevor Stanfill

    • University of Arizona

Authors

  • Trevor Stanfill

    • University of Arizona
  • John R Schaibley

    • University of Arizona
  • Brian J LeRoy

    • University of Arizona
  • Daniel Noah Shanks

    • NASA Jet Propulsion Laboratory (JPL)
  • Kenji Watanabe

    • National Institute for Materials Science
    • NIMS
    • Research Center for Functional Materials, National Institute for Materials Science
    • Research Center for Electronic and Optical Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • Research Center for Functional Materials, National Institute of Material Science, Tsukuba, Japan
    • National Institute of Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Takashi Taniguchi

    • National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute of Material Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
  • Vasili Perebeinos

    • State Univ of NY - Buffalo
  • Michael Koehler

    • University of Tennessee
  • David G Mandrus

    • University of Tennessee