Giant anomalous Hall effect in a Luttinger-compensated topological ferrimagnet UOTe

ORAL

Abstract

UOTe, a newly synthesized van der Waals layered magnet with a high Néel temperature (T_Néel ≈ 150K), has emerged as a promising material platform for studying the interplay of topology, time-reversal symmetry breaking, and strong correlations. We report that a one-dimensional (1D) atomic structure supermodulation with a periodicity of ~6.7 unit cells along the a-axis of UOTe significantly modulates its low-energy electronic properties. In longitudinal transport measurements, we observed a pronounced transport anisotropy between the a- and b-axis of the crystal. Meanwhile, transverse transport revealed a giant anomalous Hall effect accompanied by vanishingly small magnetization. Notably, the anomalous Hall angle (tan(θH) ≈ 0.2–0.4) is among the highest recorded for bulk magnetic materials. This giant anomalous Hall signal with vanishingly small magnetization suggest a Luttinger-compensated ferrimagnetic state in UOTe (where the Luttinger theorem dictates spin compensation between Uranium atoms). Here, the combination of strong spin-orbit coupling and 1D supermodulation-induced symmetry breaking leads to highly anisotropic Fermi surfaces with local Berry curvature hot spots. Finally, the robust anomalous Hall effect, combined with near-zero magnetization and a large coercive field (up to 8T at ~100K), positions UOTe as a promising candidate for spintronic applications.

*This research was supported by the Center for Advancement of Topological Semimetals, an Energy Frontier Research Center funded by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, through the Ames Laboratory under Contract No. DE-AC02-07CH11358.

Presenters

  • Thao H Dinh

    • Harvard University

Authors

  • Thao H Dinh

    • Harvard University
  • Mengke Liu

    • Harvard University
  • Sougata Mardanya

    • Howard University
  • Suk Hyun Sung

    • University of Michigan
  • Christopher Broyles

    • Washington University, St. Louis
  • Sheng Ran

    • Washington University, St. Louis
  • Ismail El Baggari

    • Harvard University
    • The Rowland Institute at Harvard
    • The Rowland Institute at Harvard, Harvard University, Cambridge, MA, USA
  • Jennifer E Hoffman

    • Harvard University
  • Sugata Chowdhury

    • Howard University
  • Kai Sun

    • University of Michigan
  • Philip Kim

    • Harvard University
  • Su-Yang Xu

    • Harvard University