Extreme magnetoresistance in γ-Al<sub>2</sub>O<sub>3</sub>/SrTiO<sub>3</sub>
ORAL
Abstract
Magnetic field-induced changes in the electrical resistance can provide a large amount of information on the electronic and magnetic structure of a studied material. A specific type of magnetoresistance, extreme magnetoresistance (XMR), is often associated with a non-saturating magnetoresistance in materials with a gapless band structure such as topological and non-topological materials.
For this work, a linear, non-saturating magnetoresistance (MR) of 80,000% at 15 T and 2 K at the high-mobility interface between the insulating γ-Al2O3 and SrTiO3 is presented. Temperature/field phase diagrams of the data revealed three crossover magnetic fields that are strongly reminiscent of the temperature/field response of semimetals displaying XMR.
Further analysis of the magnetotransport data, probing of the band structure and microscopic current imaging suggests that weak disorder provokes a squeezed guiding center motion of electrons, which induces an XMR response. Due to the dynamic origin of the high-mobility interface, the linear XMR can be tuned via redistribution of oxygen vacancies, making it an excellent candidate material for magnetic field sensing applications.
This research presents a mechanistic origin of XMR in the γ-Al2O3/SrTiO3 heterostructure and provides with an experimental pathway for employing this highly correlated heterostructure into the next generation of magnetic field sensors, using a geometric enhancement of the magnetoresistance.
For this work, a linear, non-saturating magnetoresistance (MR) of 80,000% at 15 T and 2 K at the high-mobility interface between the insulating γ-Al2O3 and SrTiO3 is presented. Temperature/field phase diagrams of the data revealed three crossover magnetic fields that are strongly reminiscent of the temperature/field response of semimetals displaying XMR.
Further analysis of the magnetotransport data, probing of the band structure and microscopic current imaging suggests that weak disorder provokes a squeezed guiding center motion of electrons, which induces an XMR response. Due to the dynamic origin of the high-mobility interface, the linear XMR can be tuned via redistribution of oxygen vacancies, making it an excellent candidate material for magnetic field sensing applications.
This research presents a mechanistic origin of XMR in the γ-Al2O3/SrTiO3 heterostructure and provides with an experimental pathway for employing this highly correlated heterostructure into the next generation of magnetic field sensors, using a geometric enhancement of the magnetoresistance.
*D.V.C. and T.S.S. acknowledge the support of Novo Nordisk FoundationNERD Programme: New Exploratory Research and Discovery, SuperiorGrant NNF21OC0068015. D.V.C., T.D.P. and N.P. acknowledge the supportof Novo Nordisk Foundation Challenge Programme 2021: Smartnanomaterials for applications in life-science, BIOMAG GrantNNF21OC0066526. N.P. acknowledges the support from the ERCAdvanced “NEXUS” Grant 101054572. B.K. acknowledges support fromERC COG no. 866236, ISF- 228/22, DIP KA 3970/1-1, and COST actionSUPERQUMAP CA 21144.
–
Presenters
-
Tristan Steegemans
- DTU Energy