Percolative phase transition in few-layered MoSe<sub>2</sub> field-effect transistors using Co and Cr contacts

ORAL

Abstract

The metal-to-insulator (MIT) phase transition in two-dimensional (2D) materials under the influence of a gating electric field has revealed interesting electronic transport phenomena. Although the mechanism of the MIT in 2D semiconductors is a topic under debate, our work addresses the tunable percolative phase transition in few-layered MoSe2 field-effect transistors (FET) with various metallic contacts. Here, we attempted to understand the MIT through temperature-dependent electronic transport measurements under the influence of an applied gate voltage. We examined the phenomenon with devices using two different kinds of metal contacts: more conventional chromium (Cr) and ferromagnetic cobalt (Co). The temperature-dependent conductivity data showed insulating-to-metallic behavior as a function of increasing carrier density, which was analyzed by fitting the data to the theory of a percolative phase transition.

*Funding for this work was provided by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences program under Award Number DE-SC0024072. Use of the Center for Nanoscale Materials, a Department of Energy Office of Science User Facility, was supported by the U.S. DOE, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by the National Science Foundation Cooperative Agreements No. DMR-1644779 and DMR-2128556 and the State of Florida.

Presenters

  • Stephen A McGill

    • National High Magnetic Field Laboratory

Authors

  • Stephen A McGill

    • National High Magnetic Field Laboratory
  • Roshan Padhan

    • Jackson State University
    • 2Layered Materials and Device Physics Laboratory, Department of Chemistry, Physics and Atmospheric Science, Jackson State University, Jackson, MS 39217, USA
  • Carlos G Garcia

    • Florida State University
  • Anirudha V Sumant

    • Argonne National Laboratory
    • Center for Nanoscale Materials, Argonne National Laboratory
  • Sujit A Kadam

    • Jackson State University
  • Ralu Divan

    • Argonne National Laboratory
    • Center for Nanoscale Materials, Argonne National Laboratory
  • Daniel Rossenmann

    • Argonne National Laboratory
  • Akshay Wali

    • Argonne National Laboratory
    • Jackson State University
  • Christina S MILLER

    • Argonne National Laboratory
  • Nihar Pradhan

    • Jackson State University
    • 2Layered Materials and Device Physics Laboratory, Department of Chemistry, Physics and Atmospheric Science, Jackson State University, Jackson, MS 39217, USA