Near-room-temperature ferromagnetic ordering in the pressure-induced collapsed-tetragonal phase in SrCo<sub>2</sub>P<sub>2</sub>

ORAL

Abstract

We present high-pressure electrical transport, magnetization, and single-crystal X-ray diffraction data on SrCo2P2. X-ray diffraction shows a transition to a collapsed tetragonal (cT) structure above ~10 GPa, with the resistance measurement revealing a clear transition-like feature up to 260 K. Magnetization, magnetoresistance, and Hall measurements indicate the transition leads to a ferromagnetic ground state. Density functional theory (DFT) calculations support a first-order transition between tetragonal and cT phases at ~10 GPa and show the emergence of ferromagnetic ordering in the cT phase. Above ~30 GPa, magnetic ordering vanishes in a first-order-like manner, consistent with theoretical predictions, suggesting SrCo2P2 is another sample of ferromagnetic intermetallic compound that avoids quantum criticality.

*Work at Ames National Laboratory is supported by the US DOE, Basic Energy Sciences, Material Science and Engineering Division under contract no. DE-AC02-07CH11358.

Presenters

  • Raquel A. Ribeiro

    • Iowa State University

Authors

  • Raquel A. Ribeiro

    • Iowa State University
  • Shuyuan huyan

    • Ames National Laboratory
  • Juan Schmidt

    • Ames National Laboratory
    • Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University
  • Juan Schmidt

    • Ames National Laboratory
    • Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University
  • Adrian Valadkhani

    • Goethe University Frankfurt
  • Haozhe Wang

    • Michigan State University
  • Zhuoqi Li

    • Ames National Laboratory
  • Aashish Sapkota

    • Ames National Laboratory
  • James L Petri

    • University of Alabama at Birmingham
  • Tyler J Slade

    • Ames National Laboratory
  • Wenli Bi

    • University of Alabama at Birmingham
  • Weiwei Xie

    • Michigan State University
  • Igor I Mazin

    • George Mason University
    • George Mason University, Quantum Science and Engineering Center
    • Depertment of Physics and Astronomy, George Mason University; Quantum Science and Engineering Centre, George Mason University
  • Roser Valenti

    • Goethe University Frankfurt
    • Frankfurt
  • Sergey L Bud'ko

    • Iowa State University
    • Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University
    • Ames National Laboratory and Iowa State University
  • Paul C Canfield

    • Iowa State University
    • Ames National Laboratory, and Department of Physics and Astronomy, Iowa State University
    • Ames National Laboratory and Iowa State University