Near-room-temperature ferromagnetic ordering in the pressure-induced collapsed-tetragonal phase in SrCo<sub>2</sub>P<sub>2</sub>
ORAL
Abstract
We present high-pressure electrical transport, magnetization, and single-crystal X-ray diffraction data on SrCo2P2. X-ray diffraction shows a transition to a collapsed tetragonal (cT) structure above ~10 GPa, with the resistance measurement revealing a clear transition-like feature up to 260 K. Magnetization, magnetoresistance, and Hall measurements indicate the transition leads to a ferromagnetic ground state. Density functional theory (DFT) calculations support a first-order transition between tetragonal and cT phases at ~10 GPa and show the emergence of ferromagnetic ordering in the cT phase. Above ~30 GPa, magnetic ordering vanishes in a first-order-like manner, consistent with theoretical predictions, suggesting SrCo2P2 is another sample of ferromagnetic intermetallic compound that avoids quantum criticality.
*Work at Ames National Laboratory is supported by the US DOE, Basic Energy Sciences, Material Science and Engineering Division under contract no. DE-AC02-07CH11358.
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Presenters
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Raquel A. Ribeiro
- Iowa State University