Isolation of individual Er quantum emitters in anatase TiO<sub>2</sub> on Si photonics

ORAL

Abstract

Defects and dopant atoms in solid state materials are a promising platform for realizing single photon sources and quantum memories, which are the basic building blocks of quantum repeaters needed for long distance quantum networks. In particular, trivalent erbium (Er3+) is of interest because it couples C-band telecom optical transitions with a spin-based memory platform. In order to produce quantum repeaters at the scale required for quantum networks it is imperative to integrate these necessary building blocks with mature and scalable semiconductor processes. In this work, we demonstrate the optical isolation of single Er3+ ions in CMOS-compatible titanium dioxide (TiO2) thin films monolithically integrated on a silicon-on-insulator photonics platform. Our results demonstrate an initial step toward the realization of a monolithically integrated and scalable quantum photonics package based on Er3+ doped thin films.

*Authors R.M.P, S. Gupta., A.S., M.K.S., and S.E.S. acknowledge support from the U.S. Department of Energy Office of Science Advanced Scientific Computing Research program under Grant No. CRADA A22112 through the Chain Reaction Innovations program at Argonne National Laboratory. Authors C.J., G.D.G., I.M., S. Guha, and A.M.D. acknowledge the Q-NEXT Quantum Center, a U.S. Department of Energy, Office of Science, National Quantum Information Science Research Center, under Award Number DE-FOA-0002253 for support. Additional materials characterization support (F. J. H.) was provided by the U.S. Department of Energy, Office of Science; Basic Energy Sciences, Materials Sciences, and Engineering Division. All electron microscopy and device fabrication were performed at the Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility, supported by the U.S. DOE, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors would like to thank D. Czaplewski, C. S. Miller, R. Divan, and L. Stan for assistance with device fabrication.

Publication: 1. Cheng Ji, Robert Pettit, et al. Isolation of individual Er quantum emitters in anatase TiO2 on Si photonics. Appl. Phys. Lett. 19; 125 (8): 084001. (2024)
2. Cheng Ji, Robert Pettit, et al. Isolation of individual Er quantum emitters in anatase TiO2 on Si photonics. arxiv.org/2406.02810

Presenters

  • Cheng Ji

    • University of Chicago

Authors

  • Cheng Ji

    • University of Chicago
  • Robert M Pettit

    • MemQ Inc.
    • memQ
  • Shobhit Gupta

    • MemQ Inc
  • Gregory D Grant

    • University of Chicago
    • University of Chicago / Argonne National Laboratory
  • Ignas Masiulionis

    • University of Chicago
  • Ananthesh Sundaresh

    • MemQ Inc
  • Skylar Deckoff–Jones

    • Memq Inc
  • Max Olberding

    • MemQ Inc
  • Manish K Singh

    • MemQ Inc
  • F. Joseph Heremans

    • Argonne Nantional Lab
    • Materials Science Division and X-ray Science Division, Argonne National Laboratory
    • Argonne National Laboratory
    • Argonne National Lab
    • University of Chicago
  • Supratik Guha

    • University of Chicago
  • Alan Michael Dibos

    • Argonne National Laboratory
  • Sean E Sullivan

    • MemQ Inc