Spectroscopic evidence of correlation and band flattening in twisted bilayer MoTe<sub>2</sub>

Oral-In-person

Abstract

Twisted bilayer MoTe2 (tMoTe2) is an emergent platform for exploring exotic quantum phases driven by the interplay between nontrivial band topology and strong electron correlations. Using angle-resolved photoemission spectroscopy (ARPES), we directly map the momentum-resolved band structure of tMoTe2 across a series of small twist angles, revealing distinct angle-dependent band reconstruction shaped by orbital character, interlayer coupling, and moiré potential modulation. This reconstruction manifests most clearly in the K-valley effective mass, which exhibits a non-monotonic evolution with twist angle, peaking near 2°, consistent with the predicted magic-angle band flattening. Complementary electrostatic gating and surface dosing further reveal the conduction band minimum, confirming tMoTe2 as a direct band gap semiconductor. These results establish a spectroscopic foundation for modeling and engineering emergent quantum phases in this moiré platform [1].

Publication: [1] Y. Deng et al., "Non-monotonic band flattening near the magic angle in twisted bilayer tMoTe2," arXiv:2509.08993 (2025).

Presenters

  • Yujun Deng

    • Stanford University

Authors

  • Yujun Deng

    • Stanford University
  • William Holtzmann

    • University of Washington
  • Ziyan Zhu

    • Boston College
  • Timothy Zaklama

    • MIT
  • Paulina Majchrzak

    • Stanford University
  • Takashi Taniguchi

    • National Institute for Materials Science
  • Kenji Watanabe

    • National Institute for Materials Science
  • Makoto Hashimoto

    • SLAC National Accelerator Laboratory
  • Donghui Lu

    • SLAC National Accelerator Laboratory
  • Christopher Jozwiak

  • Aaron Bostwick

  • Eli Rotenberg

    • Lawrence Berkeley National Laboratory
  • Liang Fu

    • Massachusetts Institute of Technology
  • Thomas Devereaux

    • Stanford University
  • Xiaodong Xu

    • University of Washington
  • Zhi-Xun Shen

    • Stanford University