Evidence for structural and electronic rare-region physics in the nickelate La<sub>2-x</sub>Sr<sub>x</sub>NiO<sub>4</sub>

ORAL

Abstract

Recent x-ray and neutron scattering measurements of the cuprate La2-xSrxCuO4 revealed an unusual exponential scaling with temperature of short-range orthorhombic correlations in the high-temperature tetragonal phase [1,2]. This scaling closely resembles the previously reported superconducting fluctuation behavior in cuprates and other oxide superconductors [3]. These observations indicate the prevalence of rare-region physics, where intrinsic inhomogeneity plays a crucial role in both the structural and electronic properties. Here we report similar behavior for La2-xSrxNiO4, a non-superconducting isostructural analogue of La2-xSrxCuO4, across a wide range of doping levels. Furthermore, we extend our investigation to spin and charge fluctuations of La2-xSrxNiO4, which reveal similar characteristics. These findings highlight the significance of rare-region effects in perovskites and related oxides.

[1] D. Pelc et al., Sci. Rep. 12, 20483 (2022)

[2] R. J. Spieker et al., arXiv:2502.02947 (2025)

[3] D. Pelc et al., Nat. Commun. 10, 2729 (2019)

*Work funded by the U.S. Department of Energy through the University of Minnesota Center for Quantum Materials, under Grant No. DE-SC0016371, and by the Croatian Science Foundation under UIP-2020-02-9494.

Publication: Evidence for rare-region physics in the structural degrees of freedom of the layered nickelate La2-xSrxNiO4. (Planned Paper)

Presenters

  • Aina Lopez Benet

    • University of Minnesota

Authors

  • Aina Lopez Benet

    • University of Minnesota
  • Richard J Spieker

    • University of Minnesota
  • Brian Krohnke

    • University of Minnesota
  • Dayu Zhai

    • University of Minnesota
  • Marin Spaić

    • University of Zagreb
  • Xing He

    • University of Pennsylvania
    • University of Minnesota
  • Chiou Yang Tan

    • University of Minnesota
  • Zachary W Anderson

    • Argonne National Laboratory, Materials Science Division
  • Feng Ye

    • Oak Ridge National Laboratory
  • Huibo Cao

    • Oak Ridge National Laboratory
  • Matthew J Krogstad

    • Argonne National Laboratory
  • Raymond Osborn

    • Argonne National Laboratory
  • Damjan Pelc

    • University of Zagreb
  • Martin Greven

    • University of Minnesota
    • University of Minnesota Twin Cities