Disorder-broadened topological Hall phase and anomalous Hall scaling in FeGe

ORAL

Abstract

Magnetic skyrmions are topologically protected spin textures whose stability and dynamics are highly sensitive to structural disorder. While defects are predicted to stabilize skyrmions through pinning, experimental studies systematically linking defect density to skyrmion phase boundaries and the underlying electron-scattering mechanisms remain scarce. Understanding these skyrmion–defect interactions is crucial for designing reliable, low-power spintronic devices. Here we systematically tune atomic-scale disorder in epitaxial B20 phase 80 nm using 400 keV Ne⁺ irradiation over fluences from 10¹¹ to 10¹⁴ ions cm⁻² and track the resulting evolution of topological and anomalous Hall responses. Increasing defect density broadens the topological Hall signal from a narrow window near 200 K in pristine films to persist down to 4 K in the most irradiated sample. Concurrently, scaling analysis of the anomalous Hall effect reveals a crossover from intrinsic Berry-curvature–dominated transport to extrinsic skew-scattering behavior with increasing defect density. Further, the skew coefficient increases threefold between the pristine and most irradiated sample. These results establish correlations between defect concentration, skyrmion phase stability, and charge-carrier scattering mechanisms, demonstrating that defect engineering provides a pathway to stabilize skyrmions in chiral magnets for next-generation spintronic architectures.

*This material is based upon work supported by the National Science Foundation under grants DMR-1905909 and DMR-2330562 at the Colorado School of Mines and the University of Washington. This work also made use of synthesis facilities at the Platform for the Accelerated Realization, Analysis, and Discovery of Interface Materials (PARADIM), which are supported by the National Science Foundation under Cooperative Agreement No. DMR-2039380. This work made use of the Cornell Center for Materials Research shared instrumentation facility. H.Y. and D.A.M. acknowledge support by the NSF Platform for the Accelerated Realization, Analysis, and Discovery of Interface Materials (PARADIM) under cooperative agreement No. DMR-2039380. The Thermo Fisher Spectra 300 X-CFEG was acquired with support from PARADIM, (NSF DMR-2039380), and Cornell University. Part of this work was performed at the Center for Integrated Nanotechnologies, a DOE Office of Science User Facility. Sandia National Laboratories, managed and operated by NTESS, LLC, a wholly owned subsidiary of Honeywell International, Inc., for the U.S. DOE’s National Nuclear Security Administration. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is managed by Triad National Security, LLC for the U.S. Department of Energy’s NNSA, under contract 89233218CNA000001. The views expressed in the article do not necessarily represent the views of the U.S. DOE or the United States Government. This work was suppor

Publication: Planned Paper: Disorder-broadened topological Hall phase and anomalous Hall scaling in FeGe - submitting in Advanced Materials

Presenters

  • Chaman Gupta

    • University of Washington

Authors

  • Chaman Gupta

    • University of Washington
  • Chris Matsumura

    • University of Washington
  • Hongbin Yang

    • Cornell University
  • Sarah P Edwards

    • University of Washington
  • Rebeca M Gurrola

    • Sandia National Laoratories
  • Jiun-Haw Chu

    • University of Washington
  • Hanjong Paik

    • University of Oklahoma
  • Yongqiang Wang

    • Los Alamos National Laboratory
  • David Anthony Muller

    • Cornell University
  • Robert Streubel

    • University of Nebraska - Lincoln
  • Tzu-Ming Lu

    • Sandia National Laboratories
  • Serena Eley

    • Department of Electrical and Computer Engineering, University of Washington; Department of Physics, Colorado School of Mines